Header logo is mms


2020


Biocompatible magnetic micro‐ and nanodevices: Fabrication of FePt nanopropellers and cell transfection
Biocompatible magnetic micro‐ and nanodevices: Fabrication of FePt nanopropellers and cell transfection

Kadiri, V. M., Bussi, C., Holle, A. W., Son, K., Kwon, H., Schütz, G., Gutierrez, M. G., Fischer, P.

Adv. Mat., 32(2001114), May 2020 (article)

Abstract
The application of nanoparticles for drug or gene delivery promises benefits in the form of single‐cell‐specific therapeutic and diagnostic capabilities. Many methods of cell transfection rely on unspecific means to increase the transport of genetic material into cells. Targeted transport is in principle possible with magnetically propelled micromotors, which allow responsive nanoscale actuation and delivery. However, many commonly used magnetic materials (e.g., Ni and Co) are not biocompatible, possess weak magnetic remanence (Fe3O4), or cannot be implemented in nanofabrication schemes (NdFeB). Here, it is demonstrated that co‐depositing iron (Fe) and platinum (Pt) followed by one single annealing step, without the need for solution processing, yields ferromagnetic FePt nanomotors that are noncytotoxic, biocompatible, and possess a remanence and magnetization that rival those of permanent NdFeB micromagnets. Active cell targeting and magnetic transfection of lung carcinoma cells are demonstrated using gradient‐free rotating millitesla fields to drive the FePt nanopropellers. The carcinoma cells express enhanced green fluorescent protein after internalization and cell viability is unaffected by the presence of the FePt nanopropellers. The results establish FePt, prepared in the L10 phase, as a promising magnetic material for biomedical applications with superior magnetic performance, especially for micro‐ and nanodevices.

link (url) DOI [BibTex]


no image
Effect of the soft layer thickness of magnetization reversal process of exchange-spring nanomagnet patterns

Son, K., Schütz, G., Goering, E.

{Current Applied Physics}, 20(4):477-483, Elsevier B.V., Amsterdam, 2020 (article)

DOI [BibTex]


{Creating zero-field skyrmions in exchange-biased multilayers through X-ray illumination}
Creating zero-field skyrmions in exchange-biased multilayers through X-ray illumination

Guang, Y., Bykova, I., Liu, Y., Yu, G., Goering, E., Weigand, M., Gräfe, J., Kim, S. K., Zhang, J., Zhang, H., Yan, Z., Wan, C., Feng, J., Wang, X., Guo, C., Wei, H., Peng, Y., Tserkovnyak, Y., Han, X., Schütz, G.

{Nature Communications}, 11, Nature Publishing Group, London, 2020 (article)

Abstract
Skyrmions, magnetic textures with topological stability, hold promises for high-density and energy-efficient information storage devices owing to their small size and low driving-current density. Precise creation of a single nanoscale skyrmion is a prerequisite to further understand the skyrmion physics and tailor skyrmion-based applications. Here, we demonstrate the creation of individual skyrmions at zero-field in an exchange-biased magnetic multilayer with exposure to soft X-rays. In particular, a single skyrmion with 100-nm size can be created at the desired position using a focused X-ray spot of sub-50-nm size. This single skyrmion creation is driven by the X-ray-induced modification of the antiferromagnetic order and the corresponding exchange bias. Furthermore, artificial skyrmion lattices with various arrangements can be patterned using X-ray. These results demonstrate the potential of accurate optical control of single skyrmion at sub-100 nm scale. We envision that X-ray could serve as a versatile tool for local manipulation of magnetic orders.

DOI [BibTex]

DOI [BibTex]


{Tuning the magnetic properties of permalloy-based magnetoplasmonic crystals for sensor applications}
Tuning the magnetic properties of permalloy-based magnetoplasmonic crystals for sensor applications

Murzin, D. V., Belyaev, V. K., Groß, F., Gräfe, J., Rivas, M., Rodionova, V. V.

{Japanese Journal of Applied Physics}, 59(SE), IOP Publishing Ltd, Bristol, England, 2020 (article)

Abstract
Miniature magnetic sensors based on magnetoplasmonic crystals (MPlCs) exhibit high sensitivity and high spatial resolution, which can be obtained by the excitation of surface plasmon polaritons. A field dependence of surface plasmon polaritons' enhanced magneto-optical response strongly correlates with magnetic properties of MPlCs that can be tuned by changing spatial parameters, such as the period and height of diffraction gratings and thicknesses of functional layers. This work compares the magnetic properties of MPlCs based on Ni80Fe20 (permalloy) obtained from local (longitudinal magneto-optical Kerr effect) and bulk (vibrating-sample magnetometry) measurements and demonstrates an ability to control sensors' performance through changing the magnetic properties of the MPlCs. The influence of the substrate's geometry (planar or sinusoidal and trapezoidal diffraction grating profiles) and the thickness of the surface layer is examined.

DOI [BibTex]

DOI [BibTex]


no image
Specific isotope-responsive breathing transition in flexible metal-organic frameworks

Kim, J. Y., Park, J., Ha, J., Jung, M., Wallacher, D., Franz, A., Balderas-Xicohténcatl, R., Hirscher, M., Kang, S. G., Park, J. T., Oh, I. H., Moon, H. R., Oh, H.

Journal of the American Chemical Society, 142(31):13278-13282, American Chemical Society, Washington, DC, 2020 (article)

DOI [BibTex]

DOI [BibTex]


no image
Element-resolved study of the evolution of magnetic response in FexN compounds

Chen, Y., Gölden, D., Dirba, I., Huang, M., Gutfleisch, O., Nagel, P., Merz, M., Schuppler, S., Schütz, G., Alff, L., Goering, E.

{Journal of Magnetism and Magnetic Materials}, 498, NH, Elsevier, Amsterdam, 2020 (article)

DOI [BibTex]

DOI [BibTex]


no image
The role of temperature and drive current in skyrmion dynamics

Litzius, K., Leliaert, J., Bassirian, P., Rodrigues, D., Kromin, S., Lemesh, I., Zazvorka, J., Lee, K., Mulkers, J., Kerber, N., Heinze, D., Keil, N., Reeve, R. M., Weigand, M., Van Waeyenberge, B., Schütz, G., Everschor-Sitte, K., Beach, G. S. D., Kläui, M.

{Nature Electronics}, 3(1):30-36, Springer Nature, London, 2020 (article)

DOI [BibTex]

DOI [BibTex]


no image
Magnetic flux penetration into micron-sized superconductor/ferromagnet bilayers

Simmendinger, J., Weigand, M., Schütz, G., Albrecht, J.

{Superconductor Science and Technology}, 33(2), IOP Pub., Bristol, 2020 (article)

DOI [BibTex]

DOI [BibTex]


no image
Demonstration of k-vector selective microscopy for nanoscale mapping of higher order spin wave modes

Träger, N., Gruszecki, P., Lisiecki, F., Groß, F., Förster, J., Weigand, M., Glowinski, H., Kuswik, P., Dubowik, J., Krawczyk, M., Gräfe, J.

Nanoscale, 12(33):17238-17244, Royal Society of Chemistry, Cambridge, UK, 2020 (article)

DOI [BibTex]

DOI [BibTex]


no image
Direct observation of spin-wave focusing by a Fresnel lens

Gräfe, J., Gruszecki, P., Zelent, M., Decker, M., Keskinbora, K., Noske, M., Gawronski, P., Stoll, H., Weigand, M., Krawczyk, M., Back, C. H., Goering, E. J., Schütz, G.

Physical Review B, 102(2), American Physical Society, Woodbury, NY, 2020 (article)

DOI [BibTex]

DOI [BibTex]


no image
Bandgap-adjustment and enhanced surface photovoltage in Y-substituted LaTaIVO2N

Bubeck, C., Widenmeyer, M., De Denko, A. T., Richter, G., Coduri, M., Salas-Colera, E., Goering, E., Zhang, H., Yoon, S., Osterloh, F. E., Weidenkaff, A.

Journal of Materials Chemistry A, 8(23):11837-11848, Royal Society of Chemistry, Cambridge, UK, 2020 (article)

DOI [BibTex]

DOI [BibTex]


no image
Fabrication and temperature-dependent magnetic properties of large-area L10-FePt/Co exchange-spring magnet nanopatterns

Son, K., Schütz, G.

{Physica E: Low-Dimensional Systems And Nanostructures}, 115, North-Holland, Amsterdam, 2020 (article)

DOI [BibTex]

DOI [BibTex]


no image
Research trend of metal-organic frameworks for magnetic refrigeration materials application

Kim, S., Son, K., Oh, H.

Korean Journal of Materials Research, 30(3):136-141, Materials Society of Korea, Seoul, 2020 (article)

DOI [BibTex]

DOI [BibTex]


Magnetic Anisotropy in Thin Layers of (Mn,Zn)Fe2O4 on SrTiO3 (001)
Magnetic Anisotropy in Thin Layers of (Mn,Zn)Fe2O4 on SrTiO3 (001)

Denecke, R., Welke, M., Huth, P., Gräfe, J., Brachwitz, K., Lorenz, M., Grundmann, M., Ziese, M., Esquinazi, P. D., Goering, E., Schütz, G., Schindler, K., Chassé, A.

Physica Status Solidi (b), 257(7):1900627, 2020 (article)

Abstract
Herein, a ferrimagnetic manganese zinc ferrite (Mn0.5Zn0.5Fe2O4) film with a thickness of 200 nm is prepared without a buffer layer on strontium titanate (001) (SrTiO3) using pulsed laser deposition. Its magnetic properties are investigated using superconducting quantum interference device (SQUID), X-ray absorption spectroscopy with subsequent X-ray magnetic circular dichroism (XMCD) and magneto-optic Kerr effect (MOKE). Hysteresis loops derived from SQUID exhibits bulk-like properties. This can further be confirmed by bulk-like XMCD spectra. In remanent magnetization, an in-plane magnetization with basically no out-of-plane component is found. The magnetic moments derived by the sum rule formalism from the XMCD data are in good agreement to the magnetization observed by SQUID and MOKE. XMCD as well as MOKE reveal an in-plane angular fourfold magnetic anisotropy with the easy direction along [110] for (Mn0.5Zn0.5)Fe2O4 on SrTiO3. The element-specific magnetic moments from XMCD show a stronger contribution of Fe to the anisotropy than of Mn and distinct contributions of the orbital moments.

link (url) DOI [BibTex]

link (url) DOI [BibTex]


no image
In situ x-ray diffraction and spectro-microscopic study of ALD protected copper films

Dogan, G., Sanli, U. T., Hahn, K., Müller, L., Gruhn, H., Silber, C., Schütz, G., Grévent, C., Keskinbora, K.

ACS Applied Materials and Interfaces, 12(29):33377-33385, American Chemical Society, Washington, DC, 2020 (article)

DOI [BibTex]

DOI [BibTex]


no image
How to functionalise metal-organic frameworks to enable guest nanocluster embedment

King, J., Zhang, L., Doszczeczko, S., Sambalova, O., Luo, H., Rohman, F., Phillips, O., Borgschulte, A., Hirscher, M., Addicoat, M., Szilágyi, P. A.

{Journal of Materials Chemistry A}, 8(9):4889-4897, Royal Society of Chemistry, Cambridge, UK, 2020 (article)

DOI [BibTex]

DOI [BibTex]


no image
Magnetic and microstructural properties of anisotropic MnBi magnets compacted by spark plasma sintering

Chen, Y., Gregori, G., Rheingans, B., Huang, W., Kronmüller, H., Schütz, G., Goering, E.

{Journal of Alloys and Compounds}, 830, Elsevier B.V., Lausanne, Switzerland, 2020 (article)

DOI [BibTex]

DOI [BibTex]


no image
Biocompatible magnetic micro- and nanodevices: Fabrication of FePt nanopropellers and cell transfection

Kadiri, V. M., Bussi, C., Holle, A. W., Son, K., Kwon, H., Schütz, G., Gutierrez, M. G., Fischer, P.

Advanced Materials, 32(25), Wiley-VCH, Weinheim, 2020 (article)

DOI [BibTex]

DOI [BibTex]


no image
Metal organic frameworks as tunable linear magnets

Son, K., Kim, R. K., Kim, S., Schütz, G., Choi, K. M., Oh, H.

Physica Status Solidi A, 217(12), Wiley-VCH, Weinheim, 2020 (article)

DOI [BibTex]

DOI [BibTex]


no image
Generation and characterization of focused helical x-ray beams

Loetgering, L., Baluktsian, M., Keskinbora, K., Horstmeyer, R., Wilhein, T., Schütz, G., Eikema, K. S. E., Witte, S.

Science Advances, 6(7), American Association for the Advancement of Science, 2020 (article)

Generation and characterization of focused helical x-ray beams link (url) DOI [BibTex]

Generation and characterization of focused helical x-ray beams link (url) DOI [BibTex]


no image
Materials for hydrogen-based energy storage - past, recent progress and future outlook

Hirscher, M., Yartys, V. A., Baricco, M., Bellosta von Colbe, J., Blanchard, D., Bowman Jr., R. C., Broom, D. P., Buckley, C. E., Chang, F., Chen, P., Cho, Y. W., Crivello, J., Cuevas, F., David, W. I. F., de Jongh, P. E., Denys, R. V., Dornheim, M., Felderhoff, M., Filinchuk, Y., Froudakis, G. E., Grant, D. M., Gray, E. M., Hauback, B. C., He, T., Humphries, T. D., Jensen, T. R., Kim, S., Kojima, Y., Latroche, M., Li, H., Lotostskyy, M. V., Makepeace, J. W., M\oller, K. T., Naheed, L., Ngene, P., Noréus, D., Nyg\aard, M. M., Orimo, S., Paskevicius, M., Pasquini, L., Ravnsbaek, D. B., Sofianos, M. V., Udovic, T. J., Vegge, T., Walker, G. S., Webb, C. J., Weidenthaler, C., Zlotea, C.

{Journal of Alloys and Compounds}, 827, Elsevier B.V., Lausanne, Switzerland, 2020 (article)

DOI [BibTex]

DOI [BibTex]


{Thermal nucleation and high-resolution imaging of submicrometer magnetic bubbles in thin thulium iron garnet films with perpendicular anisotropy}
Thermal nucleation and high-resolution imaging of submicrometer magnetic bubbles in thin thulium iron garnet films with perpendicular anisotropy

Büttner, F., Mawass, M. A., Bauer, J., Rosenberg, E., Caretta, L., Avci, C. O., Gräfe, J., Finizio, S., Vaz, C. A. F., Novakovic, N., Weigand, M., Litzius, K., Förster, J., Träger, N., Groß, F., Suzuki, D., Huang, M., Bartell, J., Kronast, F., Raabe, J., Schütz, G., Ross, C. A., Beach, G. S. D.

{Physical Review Materials}, 4(1), American Physical Society, College Park, MD, 2020 (article)

Abstract
Ferrimagnetic iron garnets are promising materials for spintronics applications, characterized by ultralow damping and zero current shunting. It has recently been found that few nm-thick garnet films interfaced with a heavy metal can also exhibit sizable interfacial spin-orbit interactions, leading to the emergence, and efficient electrical control, of one-dimensional chiral domain walls. Two-dimensional bubbles, by contrast, have so far only been confirmed in micrometer-thick films. Here, we show by high resolution scanning transmission x-ray microscopy and photoemission electron microscopy that submicrometer bubbles can be nucleated and stabilized in ∼25-nm-thick thulium iron garnet films via short heat pulses generated by electric current in an adjacent Pt strip, or by ultrafast laser illumination. We also find that quasistatic processes do not lead to the formation of a bubble state, suggesting that the thermodynamic path to reaching that state requires transient dynamics. X-ray imaging reveals that the bubbles have Bloch-type walls with random chirality and topology, indicating negligible chiral interactions at the garnet film thickness studied here. The robustness of thermal nucleation and the feasibility demonstrated here to image garnet-based devices by x-rays both in transmission geometry and with sensitivity to the domain wall chirality are critical steps to enabling the study of small spin textures and dynamics in perpendicularly magnetized thin-film garnets.

DOI [BibTex]

DOI [BibTex]


{Real-space imaging of confined magnetic skyrmion tubes}
Real-space imaging of confined magnetic skyrmion tubes

Birch, M. T., Cortés-Ortuño, D., Turnbull, L. A., Wilson, M. N., Groß, F., Träger, N., Laurenson, A., Bukin, N., Moody, S. H., Weigand, M., Schütz, G., Popescu, H., Fan, R., Steadman, P., Verezhak, J. A. T., Balakrishnan, G., Loudon, J. C., Twitchett-Harrison, A. C., Hovorka, O., Fangohr, H., Ogrin, F., Gräfe, J., Hatton, P. D.

Nature Communications, 11, pages: 1726, 2020 (article)

Abstract
Magnetic skyrmions are topologically nontrivial particles with a potential application as information elements in future spintronic device architectures. While they are commonly portrayed as two dimensional objects, in reality magnetic skyrmions are thought to exist as elongated, tube-like objects extending through the thickness of the host material. The study of this skyrmion tube state (SkT) is vital for furthering the understanding of skyrmion formation and dynamics for future applications. However, direct experimental imaging of skyrmion tubes has yet to be reported. Here, we demonstrate the real-space observation of skyrmion tubes in a lamella of FeGe using resonant magnetic x-ray imaging and comparative micromagnetic simulations, confirming their extended structure. The formation of these structures at the edge of the sample highlights the importance of confinement and edge effects in the stabilisation of the SkT state, opening the door to further investigation into this unexplored dimension of the skyrmion spin texture.

link (url) DOI [BibTex]

link (url) DOI [BibTex]


no image
Current-induced dynamical tilting of chiral domain walls in curved microwires

Finizio, S., Wintz, S., Mayr, S., Huxtable, A. J., Langer, M., Bailey, J., Burnell, G., Marrows, C. H., Raabe, J.

Applied Physics Letters, 116(18), American Institute of Physics, Melville, NY, 2020 (article)

DOI [BibTex]

DOI [BibTex]


no image
Highly effective hydrogen isotope separation through dihydrogen bond on Cu(I)-exchanged zeolites well above liquid nitrogen temperature

Xiong, R., Zhang, L., Li, P., Luo, W., Tang, T., Ao, B., Sang, G., Chen, C., Yan, X., Chen, J., Hirscher, M.

Chemical Engineering Journal, 391, Elsevier, Lausanne, 2020 (article)

DOI [BibTex]

DOI [BibTex]


no image
Ferrimagnetic skyrmions in topological insulator/ferrimagnet heterostructures

Wu, H., Groß, F., Dai, B. Q., Lujan, D., Razavi, S. A., Zhang, P., Liu, Y. X., Sobotkiewich, K., Förster, J., Weigand, M., Schütz, G., Li, X. Q., Gräfe, J., Wang, K. L.

Advanced Materials, 32(34), Wiley-VCH, Weinheim, 2020 (article)

DOI [BibTex]

DOI [BibTex]


no image
Room temperature ferromagnetism driven by Ca-doped BiFeO3 multiferroic functional material

Marzouk, M., Hashem, H. M., Soltan, S., Ramadan, A. A.

{Journal of Materials Science: Materials in Electronics}, 31(7):5599-5607, Springer, Norwell, MA, 2020 (article)

DOI [BibTex]

DOI [BibTex]

2019


Soft-magnetic coatings as possible sensors for magnetic imaging of superconductors
Soft-magnetic coatings as possible sensors for magnetic imaging of superconductors

Ionescu, A., Simmendinger, J., Bihler, M., Miksch, C., Fischer, P., Soltan, S., Schütz, G., Albrecht, J.

Supercond. Sci. and Tech., 33, pages: 015002, IOP, December 2019 (article)

Abstract
Magnetic imaging of superconductors typically requires a soft-magnetic material placed on top of the superconductor to probe local magnetic fields. For reasonable results the influence of the magnet onto the superconductor has to be small. Thin YBCO films with soft-magnetic coatings are investigated using SQUID magnetometry. Detailed measurements of the magnetic moment as a function of temperature, magnetic field and time have been performed for different heterostructures. It is found that the modification of the superconducting transport in these heterostructures strongly depends on the magnetic and structural properties of the soft-magnetic material. This effect is especially pronounced for an inhomogeneous coating consisting of ferromagnetic nanoparticles.

link (url) DOI [BibTex]

2019

link (url) DOI [BibTex]


Superior Magnetic Performance in FePt L1_0 Nanomaterials
Superior Magnetic Performance in FePt L1_0 Nanomaterials

Son, K., Ryu, G. H., Jeong, H., Fink, L., Merz, M., Nagel, P., Schuppler, S., Richter, G., Goering, E., Schütz, G.

Small, 15(1902353), July 2019 (article)

Abstract
The discovery of the high maximum energy product of 59 MGOe for NdFeB magnets is a breakthrough in the development of permanent magnets with a tremendous impact in many fields of technology. This value is still the world record, for 40 years. This work reports on a reliable and robust route to realize nearly perfectly ordered L1_0-phase FePt nanoparticles, leading to an unprecedented energy product of 80 MGOe at room temperature. Furthermore, with a 3 nm Au coverage, the magnetic polarization of these nanomagnets can be enhanced by 25% exceeding 1.8 T. This exceptional magnetization and anisotropy is confirmed by using multiple imaging and spectroscopic methods, which reveal highly consistent results. Due to the unprecedented huge energy product, this material can be envisaged as a new advanced basic magnetic component in modern micro and nanosized devices.

link (url) DOI [BibTex]

link (url) DOI [BibTex]


no image
Extracting the dynamic magnetic contrast in time-resolved X-ray transmission microscopy

Schaffers, T., Feggeler, T., Pile, S., Meckenstock, R., Buchner, M., Spoddig, D., Ney, V., Farle, M., Wende, H., Wintz, S., Weigand, M., Ohldag, H., Ollefs, K, Ney, A.

{Nanomaterials}, 9(7), MDPI, Basel, Schweiz, 2019 (article)

DOI [BibTex]

DOI [BibTex]


no image
Generation of switchable singular beams with dynamic metasurfaces

Yu, P., Li, J., Li, X., Schütz, G., Hirscher, M., Zhang, S., Liu, N.

{ACS Nano}, 13(6):7100-7106, American Chemical Society, Washington, DC, 2019 (article)

DOI [BibTex]

DOI [BibTex]


no image
Piezo-electrical control of gyration dynamics of magnetic vortices

Filianina, M., Baldrati, L., Hajiri, T., Litzius, K., Foerster, M., Aballe, L., Kläui, M.

{Applied Physics Letters}, 115(6), American Institute of Physics, Melville, NY, 2019 (article)

DOI [BibTex]

DOI [BibTex]


no image
Barely porous organic cages for hydrogen isotrope separation

Liu, M., Zhang, L., Little, M. A., Kapil, V., Ceriotti, M., Yang, S., Ding, L., Holden, D. L., Balderas-Xicohténcatl, R., He, D., Clowes, R., Chong, S. Y., Schütz, G., Chen, L., Hirscher, M., Cooper, A. I.

{Science}, 366(6465):613-620, American Association for the Advancement of Science, Washington, D.C., 2019 (article)

DOI [BibTex]

DOI [BibTex]


no image
Magnetically induced anisotropy of flux penetration into strong-pinning superconductor/ferromagnet bilayers

Simmendinger, J., Hänisch, J., Bihler, M., Ionescu, A. M., Weigand, M., Sieger, M., Hühne, R., Rijckaert, H., van Driessche, I., Schütz, G., Albrecht, J.

{New Journal of Physics}, 21, IOP Publishing, Bristol, 2019 (article)

DOI [BibTex]

DOI [BibTex]


no image
X-ray Optics Fabrication Using Unorthodox Approaches

Sanli, U., Baluktsian, M., Ceylan, H., Sitti, M., Weigand, M., Schütz, G., Keskinbora, K.

Bulletin of the American Physical Society, APS, 2019 (article)

[BibTex]

[BibTex]


{Direct observation of coherent magnons with suboptical wavelengths in a single-crystalline ferrimagnetic insulator}
Direct observation of coherent magnons with suboptical wavelengths in a single-crystalline ferrimagnetic insulator

Förster, J., Gräfe, J., Bailey, J., Finizio, S., Träger, N., Groß, F., Mayr, S., Stoll, H., Dubs, C., Surzhenko, O., Liebing, N., Woltersdorf, G., Raabe, J., Weigand, M., Schütz, G., Wintz, S.

{Physical Review B}, 100(21), American Physical Society, Woodbury, NY, 2019 (article)

Abstract
Spin-wave dynamics were studied in an extended thin film of single-crystalline yttrium iron garnet using time-resolved scanning transmission x-ray microscopy. A combination of mechanical grinding and focused ion beam milling has been utilized to achieve a soft x-ray transparent thickness of the underlying bulk gadolinium gallium garnet substrate. Damon-Eshbach type spin waves down to about 100 nm wavelength have been directly imaged in real space for varying frequencies and external magnetic fields. The dispersion relation extracted from the experimental data agreed well with theoretical predictions. A significant influence of the ion milling process on the local magnetic properties was not detected.

DOI [BibTex]

DOI [BibTex]


{Nanoscale detection of spin wave deflection angles in permalloy}
Nanoscale detection of spin wave deflection angles in permalloy

Gross, F., Träger, N., Förster, J., Weigand, M., Schütz, G., Gräfe, J.

{Applied Physics Letters}, 114(1), American Institute of Physics, Melville, NY, 2019 (article)

Abstract
Magnonics is a potential candidate for beyond CMOS and neuromorphic computing technologies with advanced phase encoded logic. However, nanoscale imaging of spin waves with full phase and magnetization amplitude information is a challenge. We show a generalized scanning transmission x-ray microscopy platform to get a complete understanding of spin waves, including the k-vector, phase, and absolute magnetization deflection angle. As an example, this is demonstrated using a 50 nm thin permalloy film where we find a maximum deflection angle of 1.5° and good agreement with the k-vector dispersion previously reported in the literature. With a spatial resolution approximately ten times better than any other methods for spin wave imaging, x-ray microscopy opens a vast range of possibilities for the observation of spin waves and various magnetic structures.

DOI [BibTex]

DOI [BibTex]


{gFORC: A graphics processing unit accelerated first-order reversal-curve calculator}
gFORC: A graphics processing unit accelerated first-order reversal-curve calculator

Groß, F., Martínez-García, J. C., Ilse, S. E., Schütz, G., Goering, E., Rivas, M., Gräfe, J.

{Journal of Applied Physics}, 126(16), AIP Publishing, New York, NY, 2019 (article)

Abstract
First-order reversal-curves have proven to be an indispensable characterization tool for physics as well as for geology. However, the conventional evaluation algorithm requires a lot of computational effort for a comparable easy task to overcome measurement noise. In this work, we present a new evaluation approach, which exploits the diversity of Fourier space to not only speed up the calculation by a factor of 1000 but also move away from the conventional smoothing factor toward real field resolution. By comparing the baseline resolution of the new and the old algorithm, we are able to deduce an analytical equation that converts the smoothing factor into field resolution, making the old and new algorithm comparable. We find excellent agreement not only for various systems of increasing complexity but also over a large range of smoothing factors. The achieved speedup enables us to calculate a large number of first-order reversal-curve diagrams with increasing smoothing factor allowing for an autocorrelation approach to find a hard criterion for the optimum smoothing factor. This previously computational prohibitive evaluation of first-order reversal-curves solves the problem of over- and undersmoothing by increasing general readability and preventing information destruction.

DOI [BibTex]

DOI [BibTex]


no image
A special issue on hydrogen-based Energy storage

Hirscher, M.

{International Journal of Hydrogen Energy}, 44, pages: 7737, Elsevier, Amsterdam, 2019 (misc)

DOI [BibTex]

DOI [BibTex]


no image
Coordinated molecule-modulated magnetic phase with metamagnetism in metal-organic frameworks

Son, K., Kim, J. Y., Schütz, G., Kang, S. G., Moon, H. R., Oh, H.

{Inorganic Chemistry}, 58(14):8895-8899, American Chemical Society, Washington, DC, 2019 (article)

DOI [BibTex]

DOI [BibTex]


no image
Scaling of intrinsic domain wall magnetoresistance with confinement in electromigrated nanocontacts

Reeve, R. M., Loescher, A., Kazemi, H., Dupé, B., Mawass, M., Winkler, T., Schönke, D., Miao, J., Litzius, K., Sedlmayr, N., Schneider, I., Sinova, J., Eggert, S., Kläui, M.

{Physical Review B}, 99(21), American Physical Society, Woodbury, NY, 2019 (article)

DOI [BibTex]

DOI [BibTex]


{Coherent excitation of heterosymmetric spin waves with ultrashort wavelengths}
Coherent excitation of heterosymmetric spin waves with ultrashort wavelengths

Dieterle, G., Förster, J., Stoll, H., Semisalova, A. S., Finizio, S., Gangwar, A., Weigand, M., Noske, M., Fähnle, M., Bykova, I., Gräfe, J., Bozhko, D. A., Musiienko-Shmarova, H. Y., Tiberkevich, V., Slavin, A. N., Back, C. H., Raabe, J., Schütz, G., Wintz, S.

{Physical Review Letters}, 122(11), American Physical Society, Woodbury, N.Y., 2019 (article)

Abstract
In the emerging field of magnonics, spin waves are foreseen as signal carriers for future spintronic information processing and communication devices, owing to both the very low power losses and a high device miniaturization potential predicted for short-wavelength spin waves. Yet, the efficient excitation and controlled propagation of nanoscale spin waves remains a severe challenge. Here, we report the observation of high-amplitude, ultrashort dipole-exchange spin waves (down to 80 nm wavelength at 10 GHz frequency) in a ferromagnetic single layer system, coherently excited by the driven dynamics of a spin vortex core. We used time-resolved x-ray microscopy to directly image such propagating spin waves and their excitation over a wide range of frequencies. By further analysis, we found that these waves exhibit a heterosymmetric mode profile, involving regions with anti-Larmor precession sense and purely linear magnetic oscillation. In particular, this mode profile consists of dynamic vortices with laterally alternating helicity, leading to a partial magnetic flux closure over the film thickness, which is explained by a strong and unexpected mode hybridization. This spin-wave phenomenon observed is a general effect inherent to the dynamics of sufficiently thick ferromagnetic single layer films, independent of the specific excitation method employed.

DOI [BibTex]

DOI [BibTex]


Reprogrammability and Scalability of Magnonic Fibonacci Quasicrystals
Reprogrammability and Scalability of Magnonic Fibonacci Quasicrystals

Lisiecki, F., Rychły, J., Kuświk, P., Głowiński, H., Kłos, J. W., Groß, F., Bykova, I., Weigand, M., Zelent, M., Goering, E. J., Schütz, G., Gubbiotti, G., Krawczyk, M., Stobiecki, F., Dubowik, J., Gräfe, J.

Physical Review Applied, 11, pages: 054003, 2019 (article)

Abstract
Magnonic crystals are systems that can be used to design and tune the dynamic properties of magnetization. Here, we focus on one-dimensional Fibonacci magnonic quasicrystals. We confirm the existence of collective spin waves propagating through the structure as well as dispersionless modes; the reprogammability of the resonance frequencies, dependent on the magnetization order; and dynamic spin-wave interactions. With the fundamental understanding of these properties, we lay a foundation for the scalable and advanced design of spin-wave band structures for spintronic, microwave, and magnonic applications.

link (url) DOI [BibTex]

link (url) DOI [BibTex]


no image
Magnetic field dependence of magnetotransport properties of MgB2/CrO2 bilayer thin films

Alzayed, N. S., Shahabuddin, M., Ramey, S. M., Soltan, S.

{Journal of Superconductivity and Novel Magnetism}, 32(8):2447-2455, Springer Science + Business Media B.V., New York, 2019 (article)

DOI [BibTex]

DOI [BibTex]


no image
Reconfigurable nanoscale spin wave majority gate with frequency-division multiplexing

Talmelli, G., Devolder, T., Träger, N., Förster, J., Wintz, S., Weigand, M., Stoll, H., Heyns, M., Schütz, G., Radu, I., Gräfe, J., Ciubotaru, F., Adelmann, C.

2019 (misc)

Abstract
Spin waves are excitations in ferromagnetic media that have been proposed as information carriers in spintronic devices with potentially much lower operation power than conventional charge-based electronics. The wave nature of spin waves can be exploited to design majority gates by coding information in their phase and using interference for computation. However, a scalable spin wave majority gate design that can be co-integrated alongside conventional Si-based electronics is still lacking. Here, we demonstrate a reconfigurable nanoscale inline spin wave majority gate with ultrasmall footprint, frequency-division multiplexing, and fan-out. Time-resolved imaging of the magnetisation dynamics by scanning transmission x-ray microscopy reveals the operation mode of the device and validates the full logic majority truth table. All-electrical spin wave spectroscopy further demonstrates spin wave majority gates with sub-micron dimensions, sub-micron spin wave wavelengths, and reconfigurable input and output ports. We also show that interference-based computation allows for frequency-division multiplexing as well as the computation of different logic functions in the same device. Such devices can thus form the foundation of a future spin-wave-based superscalar vector computing platform.

link (url) [BibTex]

link (url) [BibTex]


no image
Structural and magnetic properties of FePt-Tb alloy thin films

Schmidt, N. Y., Laureti, S., Radu, F., Ryll, H., Luo, C., d\textquotesingleAcapito, F., Tripathi, S., Goering, E., Weller, D., Albrecht, M.

{Physical Review B}, 100(6), American Physical Society, Woodbury, NY, 2019 (article)

DOI [BibTex]

DOI [BibTex]


no image
Tunable perpendicular exchange bias in oxide heterostructures

Kim, G., Khaydukov, Y., Bluschke, M., Suyolcu, Y. E., Christiani, G., Son, K., Dietl, C., Keller, T., Weschke, E., van Aken, P. A., Logvenov, G., Keimer, B.

{Physical Review Materials}, 3(8), American Physical Society, College Park, MD, 2019 (article)

DOI [BibTex]

DOI [BibTex]


Magnons in a Quasicrystal: Propagation, Extinction, and Localization of Spin Waves in Fibonacci Structures
Magnons in a Quasicrystal: Propagation, Extinction, and Localization of Spin Waves in Fibonacci Structures

Lisiecki, F., Rychły, J., Kuświk, P., Głowiński, H., Kłos, J. W., Groß, F., Träger, N., Bykova, I., Weigand, M., Zelent, M., Goering, E. J., Schütz, G., Krawczyk, M., Stobiecki, F., Dubowik, J., Gräfe, J.

Physical Review Applied, 11, pages: 054061, 2019 (article)

Abstract
Magnonic quasicrystals exceed the possibilities of spin-wave (SW) manipulation offered by regular magnonic crystals, because of their more complex SW spectra with fractal characteristics. Here, we report the direct x-ray microscopic observation of propagating SWs in a magnonic quasicrystal, consisting of dipolar coupled permalloy nanowires arranged in a one-dimensional Fibonacci sequence. SWs from the first and second band as well as evanescent waves from the band gap between them are imaged. Moreover, additional mini band gaps in the spectrum are demonstrated, directly indicating an influence of the quasiperiodicity of the system. Finally, the localization of SW modes within the Fibonacci crystal is shown. The experimental results are interpreted using numerical calculations and we deduce a simple model to estimate the frequency position of the magnonic gaps in quasiperiodic structures. The demonstrated features of SW spectra in one-dimensional magnonic quasicrystals allow utilizing this class of metamaterials for magnonics and make them an ideal basis for future applications.

link (url) DOI [BibTex]

link (url) DOI [BibTex]


{Nanoscale X-ray imaging of spin dynamics in Yttrium iron garnet}
Nanoscale X-ray imaging of spin dynamics in Yttrium iron garnet

Förster, J., Wintz, S., Bailey, J., Finizio, S., Josten, E., Meertens, D., Dubs, C., Bozhko, D. A., Stoll, H., Dieterle, G., Traeger, N., Raabe, J., Slavin, A. N., Weigand, M., Gräfe, J., Schütz, G.

Journal of Applied Physics, 126, 2019 (article)

Abstract
Time-resolved scanning transmission x-ray microscopy has been used for the direct imaging of spin-wave dynamics in a thin film yttrium iron garnet (YIG) with sub-200 nm spatial resolution. Application of this x-ray transmission technique to single-crystalline garnet films was achieved by extracting a lamella (13×5×0.185 μm3) of the liquid phase epitaxy grown YIG thin film out of a gadolinium gallium garnet substrate. Spin waves in the sample were measured along the Damon-Eshbach and backward volume directions of propagation at gigahertz frequencies and with wavelengths in a range between 200 nm and 10 μm. The results were compared to theoretical models. Here, the widely used approximate dispersion equation for dipole-exchange spin waves proved to be insufficient for describing the observed Damon-Eshbach type modes. For achieving an accurate description, we made use of the full analytical theory taking mode-hybridization effects into account.

link (url) DOI [BibTex]

link (url) DOI [BibTex]


no image
Tailoring of an unusual oxidation state in a lanthanum tantalum(IV) oxynitride via precursor microstructure design

Bubeck, C., Widenmeyer, M., Richter, G., Coduri, M., Goering, E., Yoon, S., Weidenkaff, A.

{Communications Chemistry}, 2, Springer Nature, London, 2019 (article)

DOI [BibTex]

DOI [BibTex]