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2020


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Effect of the soft layer thickness of magnetization reversal process of exchange-spring nanomagnet patterns

Son, K., Schütz, G., Goering, E.

{Current Applied Physics}, 20(4):477-483, Elsevier B.V., Amsterdam, 2020 (article)

DOI [BibTex]


{Creating zero-field skyrmions in exchange-biased multilayers through X-ray illumination}
Creating zero-field skyrmions in exchange-biased multilayers through X-ray illumination

Guang, Y., Bykova, I., Liu, Y., Yu, G., Goering, E., Weigand, M., Gräfe, J., Kim, S. K., Zhang, J., Zhang, H., Yan, Z., Wan, C., Feng, J., Wang, X., Guo, C., Wei, H., Peng, Y., Tserkovnyak, Y., Han, X., Schütz, G.

{Nature Communications}, 11, Nature Publishing Group, London, 2020 (article)

Abstract
Skyrmions, magnetic textures with topological stability, hold promises for high-density and energy-efficient information storage devices owing to their small size and low driving-current density. Precise creation of a single nanoscale skyrmion is a prerequisite to further understand the skyrmion physics and tailor skyrmion-based applications. Here, we demonstrate the creation of individual skyrmions at zero-field in an exchange-biased magnetic multilayer with exposure to soft X-rays. In particular, a single skyrmion with 100-nm size can be created at the desired position using a focused X-ray spot of sub-50-nm size. This single skyrmion creation is driven by the X-ray-induced modification of the antiferromagnetic order and the corresponding exchange bias. Furthermore, artificial skyrmion lattices with various arrangements can be patterned using X-ray. These results demonstrate the potential of accurate optical control of single skyrmion at sub-100 nm scale. We envision that X-ray could serve as a versatile tool for local manipulation of magnetic orders.

DOI [BibTex]

DOI [BibTex]


{Tuning the magnetic properties of permalloy-based magnetoplasmonic crystals for sensor applications}
Tuning the magnetic properties of permalloy-based magnetoplasmonic crystals for sensor applications

Murzin, D. V., Belyaev, V. K., Groß, F., Gräfe, J., Rivas, M., Rodionova, V. V.

{Japanese Journal of Applied Physics}, 59(SE), IOP Publishing Ltd, Bristol, England, 2020 (article)

Abstract
Miniature magnetic sensors based on magnetoplasmonic crystals (MPlCs) exhibit high sensitivity and high spatial resolution, which can be obtained by the excitation of surface plasmon polaritons. A field dependence of surface plasmon polaritons' enhanced magneto-optical response strongly correlates with magnetic properties of MPlCs that can be tuned by changing spatial parameters, such as the period and height of diffraction gratings and thicknesses of functional layers. This work compares the magnetic properties of MPlCs based on Ni80Fe20 (permalloy) obtained from local (longitudinal magneto-optical Kerr effect) and bulk (vibrating-sample magnetometry) measurements and demonstrates an ability to control sensors' performance through changing the magnetic properties of the MPlCs. The influence of the substrate's geometry (planar or sinusoidal and trapezoidal diffraction grating profiles) and the thickness of the surface layer is examined.

DOI [BibTex]

DOI [BibTex]


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Element-resolved study of the evolution of magnetic response in FexN compounds

Chen, Y., Gölden, D., Dirba, I., Huang, M., Gutfleisch, O., Nagel, P., Merz, M., Schuppler, S., Schütz, G., Alff, L., Goering, E.

{Journal of Magnetism and Magnetic Materials}, 498, NH, Elsevier, Amsterdam, 2020 (article)

DOI [BibTex]

DOI [BibTex]


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The role of temperature and drive current in skyrmion dynamics

Litzius, K., Leliaert, J., Bassirian, P., Rodrigues, D., Kromin, S., Lemesh, I., Zazvorka, J., Lee, K., Mulkers, J., Kerber, N., Heinze, D., Keil, N., Reeve, R. M., Weigand, M., Van Waeyenberge, B., Schütz, G., Everschor-Sitte, K., Beach, G. S. D., Kläui, M.

{Nature Electronics}, 3(1):30-36, Springer Nature, London, 2020 (article)

DOI [BibTex]

DOI [BibTex]


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Magnetic flux penetration into micron-sized superconductor/ferromagnet bilayers

Simmendinger, J., Weigand, M., Schütz, G., Albrecht, J.

{Superconductor Science and Technology}, 33(2), IOP Pub., Bristol, 2020 (article)

DOI [BibTex]

DOI [BibTex]


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Interaction of hydrogen isotopes with flexible metal-organic frameworks

Bondorf, L.

Universität Stuttgart, Stuttgart, 2020 (mastersthesis)

[BibTex]

[BibTex]


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Fabrication and temperature-dependent magnetic properties of large-area L10-FePt/Co exchange-spring magnet nanopatterns

Son, K., Schütz, G.

{Physica E: Low-Dimensional Systems And Nanostructures}, 115, North-Holland, Amsterdam, 2020 (article)

DOI [BibTex]

DOI [BibTex]


Magnetic Anisotropy in Thin Layers of (Mn,Zn)Fe2O4 on SrTiO3 (001)
Magnetic Anisotropy in Thin Layers of (Mn,Zn)Fe2O4 on SrTiO3 (001)

Denecke, R., Welke, M., Huth, P., Gräfe, J., Brachwitz, K., Lorenz, M., Grundmann, M., Ziese, M., Esquinazi, P. D., Goering, E., Schütz, G., Schindler, K., Chassé, A.

physica status solidi (b), n/a(n/a):1900627, 2020 (article)

Abstract
Herein, a ferrimagnetic manganese zinc ferrite (Mn0.5Zn0.5Fe2O4) film with a thickness of 200 nm is prepared without a buffer layer on strontium titanate (001) (SrTiO3) using pulsed laser deposition. Its magnetic properties are investigated using superconducting quantum interference device (SQUID), X-ray absorption spectroscopy with subsequent X-ray magnetic circular dichroism (XMCD) and magneto-optic Kerr effect (MOKE). Hysteresis loops derived from SQUID exhibits bulk-like properties. This can further be confirmed by bulk-like XMCD spectra. In remanent magnetization, an in-plane magnetization with basically no out-of-plane component is found. The magnetic moments derived by the sum rule formalism from the XMCD data are in good agreement to the magnetization observed by SQUID and MOKE. XMCD as well as MOKE reveal an in-plane angular fourfold magnetic anisotropy with the easy direction along [110] for (Mn0.5Zn0.5)Fe2O4 on SrTiO3. The element-specific magnetic moments from XMCD show a stronger contribution of Fe to the anisotropy than of Mn and distinct contributions of the orbital moments.

link (url) DOI [BibTex]

link (url) DOI [BibTex]


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How to functionalise metal-organic frameworks to enable guest nanocluster embedment

King, J., Zhang, L., Doszczeczko, S., Sambalova, O., Luo, H., Rohman, F., Phillips, O., Borgschulte, A., Hirscher, M., Addicoat, M., Szilágyi, P. A.

{Journal of Materials Chemistry A}, 8(9):4889-4897, Royal Society of Chemistry, Cambridge, UK, 2020 (article)

DOI [BibTex]

DOI [BibTex]


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Magnetic and microstructural properties of anisotropic MnBi magnets compacted by spark plasma sintering

Chen, Y., Gregori, G., Rheingans, B., Huang, W., Kronmüller, H., Schütz, G., Goering, E.

{Journal of Alloys and Compounds}, 830, Elsevier B.V., Lausanne, Switzerland, 2020 (article)

DOI [BibTex]

DOI [BibTex]


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Generation and characterization of focused helical x-ray beams

Loetgering, L., Baluktsian, M., Keskinbora, K., Horstmeyer, R., Wilhein, T., Schütz, G., Eikema, K. S. E., Witte, S.

Science Advances, 6(7), American Association for the Advancement of Science, 2020 (article)

Generation and characterization of focused helical x-ray beams link (url) DOI [BibTex]

Generation and characterization of focused helical x-ray beams link (url) DOI [BibTex]


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Materials for hydrogen-based energy storage - past, recent progress and future outlook

Hirscher, M., Yartys, V. A., Baricco, M., Bellosta von Colbe, J., Blanchard, D., Bowman Jr., R. C., Broom, D. P., Buckley, C. E., Chang, F., Chen, P., Cho, Y. W., Crivello, J., Cuevas, F., David, W. I. F., de Jongh, P. E., Denys, R. V., Dornheim, M., Felderhoff, M., Filinchuk, Y., Froudakis, G. E., Grant, D. M., Gray, E. M., Hauback, B. C., He, T., Humphries, T. D., Jensen, T. R., Kim, S., Kojima, Y., Latroche, M., Li, H., Lotostskyy, M. V., Makepeace, J. W., M\oller, K. T., Naheed, L., Ngene, P., Noréus, D., Nyg\aard, M. M., Orimo, S., Paskevicius, M., Pasquini, L., Ravnsbaek, D. B., Sofianos, M. V., Udovic, T. J., Vegge, T., Walker, G. S., Webb, C. J., Weidenthaler, C., Zlotea, C.

{Journal of Alloys and Compounds}, 827, Elsevier B.V., Lausanne, Switzerland, 2020 (article)

DOI [BibTex]

DOI [BibTex]


{Thermal nucleation and high-resolution imaging of submicrometer magnetic bubbles in thin thulium iron garnet films with perpendicular anisotropy}
Thermal nucleation and high-resolution imaging of submicrometer magnetic bubbles in thin thulium iron garnet films with perpendicular anisotropy

Büttner, F., Mawass, M. A., Bauer, J., Rosenberg, E., Caretta, L., Avci, C. O., Gräfe, J., Finizio, S., Vaz, C. A. F., Novakovic, N., Weigand, M., Litzius, K., Förster, J., Träger, N., Groß, F., Suzuki, D., Huang, M., Bartell, J., Kronast, F., Raabe, J., Schütz, G., Ross, C. A., Beach, G. S. D.

{Physical Review Materials}, 4(1), American Physical Society, College Park, MD, 2020 (article)

Abstract
Ferrimagnetic iron garnets are promising materials for spintronics applications, characterized by ultralow damping and zero current shunting. It has recently been found that few nm-thick garnet films interfaced with a heavy metal can also exhibit sizable interfacial spin-orbit interactions, leading to the emergence, and efficient electrical control, of one-dimensional chiral domain walls. Two-dimensional bubbles, by contrast, have so far only been confirmed in micrometer-thick films. Here, we show by high resolution scanning transmission x-ray microscopy and photoemission electron microscopy that submicrometer bubbles can be nucleated and stabilized in ∼25-nm-thick thulium iron garnet films via short heat pulses generated by electric current in an adjacent Pt strip, or by ultrafast laser illumination. We also find that quasistatic processes do not lead to the formation of a bubble state, suggesting that the thermodynamic path to reaching that state requires transient dynamics. X-ray imaging reveals that the bubbles have Bloch-type walls with random chirality and topology, indicating negligible chiral interactions at the garnet film thickness studied here. The robustness of thermal nucleation and the feasibility demonstrated here to image garnet-based devices by x-rays both in transmission geometry and with sensitivity to the domain wall chirality are critical steps to enabling the study of small spin textures and dynamics in perpendicularly magnetized thin-film garnets.

DOI [BibTex]

DOI [BibTex]


{Real-space imaging of confined magnetic skyrmion tubes}
Real-space imaging of confined magnetic skyrmion tubes

Birch, M. T., Cortés-Ortuño, D., Turnbull, L. A., Wilson, M. N., Groß, F., Träger, N., Laurenson, A., Bukin, N., Moody, S. H., Weigand, M., Schütz, G., Popescu, H., Fan, R., Steadman, P., Verezhak, J. A. T., Balakrishnan, G., Loudon, J. C., Twitchett-Harrison, A. C., Hovorka, O., Fangohr, H., Ogrin, F., Gräfe, J., Hatton, P. D.

Nature Communications, 11, pages: 1726, 2020 (article)

Abstract
Magnetic skyrmions are topologically nontrivial particles with a potential application as information elements in future spintronic device architectures. While they are commonly portrayed as two dimensional objects, in reality magnetic skyrmions are thought to exist as elongated, tube-like objects extending through the thickness of the host material. The study of this skyrmion tube state (SkT) is vital for furthering the understanding of skyrmion formation and dynamics for future applications. However, direct experimental imaging of skyrmion tubes has yet to be reported. Here, we demonstrate the real-space observation of skyrmion tubes in a lamella of FeGe using resonant magnetic x-ray imaging and comparative micromagnetic simulations, confirming their extended structure. The formation of these structures at the edge of the sample highlights the importance of confinement and edge effects in the stabilisation of the SkT state, opening the door to further investigation into this unexplored dimension of the skyrmion spin texture.

link (url) DOI [BibTex]

link (url) DOI [BibTex]


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Room temperature ferromagnetism driven by Ca-doped BiFeO3 multiferroic functional material

Marzouk, M., Hashem, H. M., Soltan, S., Ramadan, A. A.

{Journal of Materials Science: Materials in Electronics}, 31(7):5599-5607, Springer, Norwell, MA, 2020 (article)

DOI [BibTex]

DOI [BibTex]

2011


The Oxidation of Fe(111)
The Oxidation of Fe(111)

Davies, R., Edwards, D., Gräfe, J., Gilbert, L., Davies, P., Hutchings, G., Bowker, M.

Surface Science, 605(17-18):1754-1762, 2011 (article)

Abstract
The oxidation of Fe(111) was studied using Auger electron spectroscopy (AES), low energy electron diffraction (LEED), X-ray photoelectron spectroscopy (XPS), ion scattering spectroscopy (ISS) and scanning tunnelling microscopy (STM). Oxidation of the crystal was found to be a very fast process, even at 200 K, and the Auger O signal saturation level is reached within ~ 50 × 10− 6 mbar s. Annealing the oxidised surface at 773 K causes a significant decline in apparent surface oxygen concentration and produces a clear (6 × 6) LEED pattern, whereas after oxidation at ambient temperature no pattern was observed. STM results indicate that the oxygen signal was reduced due to the nucleation of large, but sparsely distributed oxide islands, leaving mainly the smooth (6 × 6) structure between the islands. The reactivity of the (6 × 6) layer towards methanol was investigated using temperature programmed desorption (TPD), which showed mainly decomposition to CO and CO2, due to the production of formate intermediates on the surface. Interestingly, this removes the (6 × 6) structure by reduction, but it can be reformed from the sink of oxygen present in the large oxide islands simply by annealing at 773 K for a few minutes. The (6 × 6) appears to be a relatively stable, pseudo-oxide phase, that may be useful as a model oxide surface.

DOI [BibTex]

2011

DOI [BibTex]


High-resolution x-ray absorption spectroscopy of BaTiO${}_{3}$: Experiment and first-principles calculations
High-resolution x-ray absorption spectroscopy of BaTiO_3: Experiment and first-principles calculations

Chassé, A., Borek, S., Schindler, K., Trautmann, M., Huth, M., Steudel, F., Makhova, L., Gräfe, J., Denecke, R.

Physical Review B, 84, pages: 195135, 2011 (article)

Abstract
High resolution x-ray absorption spectroscopy (XAS) affords new insight into the microscopic properties of perovskite transition metal oxides. Interpretation of XAS spectra in transition metal oxides requires theoretical tools capable of describing relativistic and many-body effects. In this work, full relativistic (SPR-KKR) and multiplet calculations (CTM4XAS) are carried out and compared to experimental multiedge XAS spectra of BaTiO3 single crystals. The impact of relativistic and many-body effects on the calculated density of states and x-ray absorption near edge structure spectra are individually considered.

DOI [BibTex]

DOI [BibTex]


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Ferromagnetism of ZnO influenced by physical and chemical treatment

Chen, Y.

Universität Stuttgart, Stuttgart, 2011 (mastersthesis)

[BibTex]

[BibTex]


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Herstellung und Charakterisierung von ultradünnen, funktionellen CoFeB Filmen

Streckenbach, F.

Hochschule Esslingen / Hochschule Aalen, Esslingen / Aalen, 2011 (mastersthesis)

[BibTex]

[BibTex]


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Hydrogen adsorption on metal-organic frameworks

Streppel, B.

Universität Stuttgart, Stuttgart, 2011 (phdthesis)

link (url) [BibTex]

link (url) [BibTex]


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Electron theory of fast and ultrafast dissipative magnetization dynamics

Fähnle, M., Illg, C.

{Journal of Physics: Condensed Matter}, 23, 2011 (article)

DOI [BibTex]

DOI [BibTex]


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Large-area hard magnetic L10-FePt nanopatterns by nanoimprint lithography

Bublat, T., Goll, D.

{Nanotechnology}, 22(31), 2011 (article)

DOI [BibTex]


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Hydrogen storage by cryoadsorption in ultrahigh-porosity metal-organic frameworks

Hirscher, M.

{Angewandte Chemie International Edition}, 50(3):581-582, 2011 (article)

DOI [BibTex]

DOI [BibTex]


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Amorphous grain boundary layers in the ferromagnetic nanograined ZnO films

Straumal, B. B., Mazilkin, A. A., Protasova, S. G., Myatiev, A. A., Straumal, P. B., Goering, E., Baretzky, B.

In {Thin Solid Films}, 520, pages: 1192-1194, Hersonissos, Greece, 2011 (inproceedings)

DOI [BibTex]

DOI [BibTex]


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Multilayer Fresnel zone plate for soft X-ray microscopy resolves sub-39 nm structures

Mayer, M., Grévent, C., Szeghalmi, A., Knez, M., Weigand, M., Rehbein, S., Schneider, G., Baretzky, B., Schütz, G.

{Ultramicroscopy}, 111, pages: 1706-1711, 2011 (article)

DOI [BibTex]

DOI [BibTex]


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Generalized Gilbert equation including inertial damping: derivation from an extended breathing Fermi surface model

Fähnle, M., Steiauf, D., Illg, C.

{Physical Review B}, 84, 2011 (article)

DOI [BibTex]


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Hydrogen physisorption in high SSA microporous materials - A comparison between AX-21\textunderscore33 and MOF-177 at cryogenic conditions

Schlichtenmayer, M., Streppel, B., Hirscher, M.

{International Journal of Hydrogen Energy}, 36, pages: 586-591, 2011 (article)

DOI [BibTex]

DOI [BibTex]


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Inversed solid-phase grain boundary wetting in the Al-Zn system

Protasova, S. G., Kogtenkova, O. A., Straumal, B. B., Zieba, P., Baretzky, B.

In {Interface Science Issue}, 46, pages: 4349-4353, Mie, Japan, 2011 (inproceedings)

DOI [BibTex]

DOI [BibTex]


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Magnetic vortex core reversal by excitation of spin waves

Kammerer, M., Weigand, M., Curcic, M., Noske, M., Sproll, M., Vansteenkiste, A., Van Waeyenberge, B., Stoll, H., Woltersdorf, G., Back, C. H., Schütz, G.

{Nature Communications}, 2, pages: 279-284, 2011 (article)

DOI [BibTex]

DOI [BibTex]


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Piezo driven strain effects on magneto-crystalline anisotropy

Badr, E.

Universität Stuttgart, Stuttgart, 2011 (mastersthesis)

[BibTex]

[BibTex]


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Magnetooptische Untersuchungen an granularen und beschichteten MgB2 Filmen

Stahl, C.

Universität Stuttgart, Stuttgart, 2011 (mastersthesis)

[BibTex]

[BibTex]


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Mikromagnetismus der Wechselwirkung von Spinwellen mit Domänenwänden in Ferromagneten

Macke, S.

Universität Stuttgart, Stuttgart, 2011 (phdthesis)

[BibTex]

[BibTex]


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Magnetism studied with circularly polarized X-rays

Schütz, G., Goering, E., Stoll, H.

{International Journal of Materials Research}, 102(7):773-783, 2011 (article)

DOI [BibTex]

DOI [BibTex]


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Coupled vortex oscillations in spatially separated permalloy squares

Vogel, A., Kamionka, T., Martens, M., Drews, A., Chou, K., Tyliszczak, T., Stoll, H., Van Waeyenberge, B., Meier, G.

{Physical Review Letters}, 106, 2011 (article)

DOI [BibTex]

DOI [BibTex]


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Contruction of basis functions with crystal symmetry for the spin-cluster expansion of the magnetic energy on the atomic scale

Dietermann, F., Singer, R., Fähnle, M.

{Journal of Mathematical Physics}, 52, 2011 (article)

DOI [BibTex]

DOI [BibTex]


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Magnetic patterning perpendicular anisotropy FePd alloy films by masked ion irradiation

Merkel, D. G., Bottyán, L., Tanczikó, F., Zolnai, Z., Nagy, N., Vértesy, G., Waizinger, J., Bommer, L.

{Journal of Applied Physics}, 109(12), 2011 (article)

DOI [BibTex]

DOI [BibTex]


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Stability of the current-carrying state in nonhomogeneous MgB2 films

Treiber, S., Stahl, C., Schütz, G., Albrecht, J.

{Physical Review B}, 84, 2011 (article)

DOI [BibTex]

DOI [BibTex]


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First measurement of the heat effect of the grain boundary wetting phase transition

Straumal, B. B., Kogtenkova, O. A., Protasova, S. G., Zieba, P., Czeppe, T., Baretzky, B., Valiev, R. Z.

In {Interface Science Issue}, 46, pages: 4243, Mie, Japan, 2011 (inproceedings)

DOI [BibTex]

DOI [BibTex]


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Orbital reflectometry of oxide heterostructures

Benckiser, E., Haverkort, M. W., Brück, S., Goering, E., Macke, S., Fraño, A., Yang, X., Andersen, O. K., Cristiani, G., Habermeier, H., Boris, A. V., Zegkinoglou, I., Wochner, P., Kim, H., Hinkov, V., Keimer, B.

{Nature Materials}, 10(3):189-193, 2011 (article)

DOI [BibTex]

DOI [BibTex]


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Potential explanation of charge response of magnetization in nanoporous systems

Subkow, S., Fähnle, M.

{Physical Review B}, 84, 2011 (article)

DOI [BibTex]

DOI [BibTex]


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Herstellung und Qualifizierung gesputterter Magnesiumdiboridschichten

Breyer, F.

Hochschule Aalen, Aalen, 2011 (mastersthesis)

[BibTex]

[BibTex]


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Large hidden orbital moments in magnetite

Goering, E.

{Physica Status Solidi B}, 248(10):2345-2351, 2011 (article)

DOI [BibTex]

DOI [BibTex]


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Cr magnetization reversal at the CrO2/RuO2 interface: Origin of the reduced GMR effect

Zafar, K., Audehm, P., Schütz, G., Goering, E., Pathak, M., Chetry, K. B., LeClair, P. R., Gupta, A.

{Physical Review B}, 84, 2011 (article)

DOI [BibTex]

DOI [BibTex]


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Magnetocaloric effect, magnetic domain structure and spin-reorientation transitios in HoCo5 single crystals

Skokov, K. P., Pastushenkov, Y. G., Koshkid\textquotesingleko, Y. S., Schütz, G., Goll, D., Ivanova, T. I., Nikitin, S. A., Semenova, E. M., Petrenko, A. V.

{Journal of Magnetism and Magnetic Materials}, 323(5):447-450, 2011 (article)

DOI [BibTex]

DOI [BibTex]


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Elucidating gating effects for hydrogen sorption in MFU-4-type triazolate-based metal-organic frameworks featuring different pore sizes

Denysenko, D., Grzywa, M., Tonigold, M., Streppel, B., Krkljus, I., Hirscher, M., Mugnaioli, E., Kolb, U., Hanss, J., Volkmer, D.

{Chemistry - A European Journal}, 17(6):1837-1848, 2011 (article)

DOI [BibTex]

DOI [BibTex]


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BET specific surface area and pore structure of MOFs determined by hydrogen adsorption at 20 K

Streppel, B., Hirscher, M.

{Physical Chemistry Chemical Physics}, 13(8):3220-3222, 2011 (article)

DOI [BibTex]

DOI [BibTex]


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High contrast magnetic and nonmagnetic sample current microscopy for bulk and transparent samples using soft X-rays

Nolle, D., Weigand, M., Schütz, G., Goering, E.

{Microscopy and Microanalysis}, 17, pages: 834-842, 2011 (article)

DOI [BibTex]