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2017


{Temperature-dependent first-order reversal curve measurements on unusually hard magnetic low-temperature phase of MnBi}
Temperature-dependent first-order reversal curve measurements on unusually hard magnetic low-temperature phase of MnBi

Muralidhar, S., Gräfe, J., Chen, Y., Etter, M., Gregori, G., Ener, S., Sawatzki, S., Hono, K., Gutfleisch, O., Kronmüller, H., Schütz, G., Goering, E. J.

{Physical Review B}, 95(2), American Physical Society, Woodbury, NY, 2017 (article)

Abstract
We have performed first-order reversal curve (FORC) measurements to investigate the irreversible magnetization processes in the low-temperature phase of MnBi. Using temperature-dependent FORC analysis, we are able to provide a clear insight into the effects of microstructural parameters such as grain diameter, shape, and surface composition on the coercivity of nucleation hardened permanent magnet MnBi. FORC diagrams of MnBi show a unique broadening and narrowing of the coercive field distribution with increasing temperature. We were able to microscopically identify the reason for this behavior, based on the shift in the single domain critical diameter from nearly 1 to 2 μm, thereby changing the dependence of coercivity with particle size. This is based on a strong increase in the uniaxial anisotropy constant with increasing temperature. Furthermore, the results also give an additional confirmation that the magnetic hardening in low-temperature phase MnBi occurs due to nucleation mechanisms. In our case, we show that temperature-dependent FORC measurements provide a powerful tool for the microscopic understanding of high-performance permanent magnet systems.

DOI Project Page [BibTex]

2017

DOI Project Page [BibTex]


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Exploiting diffusion barrier and chemical affinity of metal-organic frameworks for efficient hydrogen isotope separation

Kim, J. Y., Balderas-Xicohténcatl, R., Zhang, L., Kang, S. G., Hirscher, M., Oh, H., Moon, H. R.

{Journal of the American Chemical Society}, 139(42):15135-15141, American Chemical Society, Washington, DC, 2017 (article)

DOI [BibTex]

DOI [BibTex]


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Facile fabrication of mesoporous silica micro-jets with multi-functionalities

Vilela, D., Hortelao, A. C., Balderas-Xicohténcatl, R., Hirscher, M., Hahn, K., Ma, X., Sánchez, S.

{Nanoscale}, 9(37):13990-13997, Royal Society of Chemistry, Cambridge, UK, 2017 (article)

DOI [BibTex]

DOI [BibTex]


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Functionalised metal-organic frameworks: a novel approach to stabilising single metal atoms

Szilágyi, P. Á., Rogers, D. M., Zaiser, I., Callini, E., Turner, S., Borgschulte, A., Züttel, A., Geerlings, H., Hirscher, M., Dam, B.

{Journal of Materials Chemistry A}, 5(30):15559-15566, Royal Society of Chemistry, Cambridge, UK, 2017 (article)

DOI [BibTex]

DOI [BibTex]


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Selective hydrogen isotope separation via breathing transition in MIL-53(Al)

Kim, J. Y., Zhang, L., Balderas-Xicohténcatl, R., Park, J., Hirscher, M., Moon, H. R., Oh, H.

{Journal of the American Chemical Society}, 139(49):17743-17746, American Chemical Society, Washington, DC, 2017 (article)

DOI [BibTex]

DOI [BibTex]


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Efficient synthesis for large-scale production and characterization for hydrogen storage of ligand exchanged MOF-74/174/184-M (M\textequalsMg2+, Ni2+)

Oh, H., Maurer, S., Balderas-Xicohténcatl, R., Arnold, L., Magdysyuk, O. V., Schütz, G., Müller, U., Hirscher, M.

{International Journal of Hydrogen Energy}, 42(2):1027-1035, Elsevier, Amsterdam, 2017 (article)

DOI [BibTex]

DOI [BibTex]


{Advanced magneto-optical Kerr effect measurements of superconductors at low temperatures}
Advanced magneto-optical Kerr effect measurements of superconductors at low temperatures

Stahl, C., Gräfe, J., Ruoß, S., Zahn, P., Bayer, J., Simmendinger, J., Schütz, G., Albrecht, J.

{AIP Advances}, 7(10), 2017 (article)

Abstract
Magneto-optical Kerr-effect (MOKE) measurements of superconducting films with soft-magnetic coatings are performed at low temperatures using a laser-based MOKE set-up. An elaborate measurement scheme with internal reference allows the quantitative comparison of the temperature dependent Kerr-amplitude with the magnetic field generated by supercurrents. For this purpose, an amorphous CoFeB thin film exhibiting a large Kerr-signal is deposited directly on top of the YBCO superconductor acting as field sensing layer. It is shown that the resulting magnetic hysteresis loops of the soft-magnetic film can be used to reconstruct the electric properties of the superconductor.

DOI [BibTex]

DOI [BibTex]


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Corrosion-protected hybrid nanoparticles

Jeong, H., Alarcón-Correa, M., Mark, A. G., Son, K., Lee, T., Fischer, P.

{Advanced Science}, 4(12), Wiley-VCH, Weinheim, 2017 (article)

DOI [BibTex]

DOI [BibTex]


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Investigation of the Dzyaloshinskii-Moriya interaction and room temperature skyrmions in W/CoFeB/MgO thin films and microwires

Jaiswal, S., Litzius, K., Lemesh, I., Büttner, F., Finizio, S., Raabe, J., Weigand, M., Lee, K., Langer, J., Ocker, B., Jakob, G., Beach, G. S. D., Kläui, M.

{Applied Physics Letters}, 111(2), American Institute of Physics, Melville, NY, 2017 (article)

DOI [BibTex]

DOI [BibTex]


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Ultrafast demagnetization after femtosecond laser pulses: Transfer of angular momentum from the electronic system to magnetoelastic spin-phonon modes

Fähnle, M., Tsatsoulis, T., Illg, C., Haag, M., Müller, B. Y., Zhang, L.

{Journal of Superconductivity and Novel Magnetism}, 30(5):1381-1387, Springer Science + Business Media B.V., New York, 2017 (article)

DOI [BibTex]

DOI [BibTex]


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Magnetic behavior of single chain magnets in metal organic frameworks CPO-27-Co

Son, K., Goering, E., Hirscher, M., Oh, H.

{Journal of Nanoscience and Nanotechnology}, 17(10):7541-7546, American Scientific Publishers, Stevenson Ranch, Calif., 2017 (article)

DOI [BibTex]

DOI [BibTex]


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Switching by domain-wall automotion in asymmetric ferromagnetic rings

Mawass, M., Richter, K., Bisig, A., Reeve, R. M., Krüger, B., Weigand, M., Stoll, H., Krone, A., Kronast, F., Schütz, G., Kläui, M.

{Physical Review Applied}, 7(4), American Physical Society, College Park, Md. [u.a.], 2017 (article)

DOI [BibTex]

DOI [BibTex]


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A neutral atom moving in an external magnetic field does not feel a Lorentz force

Fähnle, M.

{American Journal of Modern Physics}, 6(6):153-155, Science Publishing Group, New York, NY, 2017 (article)

DOI [BibTex]

DOI [BibTex]


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Smooth and rapid microwave synthesis of MIL-53(Fe) including superparamagnetic \textlessgamma\textgreater-Fe2O3 nanoparticles

Wengert, S., Albrecht, J., Ruoß, S., Stahl, C., Schütz, G., Schäfer, R.

{Journal of Magnetism and Magnetic Materials}, 444, pages: 168-172, NH, Elsevier, Amsterdam, 2017 (article)

DOI [BibTex]

DOI [BibTex]


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Characterization and differentiation of rock varnish types from different environments by microanalytical techniques

Macholdt, D. S., Jochum, K. P., Pöhlker, C., Arangio, A., Förster, J., Stoll, B., Weis, U., Weber, B., Müller, M., Kappl, M., Shiraiwa, M., Kilcoyne, A. L. D., Weigand, M., Scholz, D., Haug, G. H., Al-Amri, A., Andreae, M. O.

{Chemical Geology}, 459, pages: 91-118, Elsevier, Amsterdam, 2017 (article)

DOI [BibTex]

DOI [BibTex]


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Skyrmion Hall effect revealed by direct time-resolved X-ray microscopy

Litzius, K., Lemesh, I., Krüger, B., Bassirian, P., Caretta, L., Richter, K., Büttner, F., Sato, K., Tretiakov, O. A., Förster, J., Reeve, R. M., Weigand, M., Bykova, I., Stoll, H., Schütz, G., Beach, G. S. D., Kläui, M.

{Nature Physics}, 13(2):170-175, Nature Pub. Group, London, 2017 (article)

DOI [BibTex]

DOI [BibTex]


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Comment on magnonic black holes

Fähnle, M., Schütz, G.

{Journal of Magnetism and Magnetic Materials}, 444, pages: 146-146, NH, Elsevier, Amsterdam, 2017 (article)

DOI [BibTex]

DOI [BibTex]


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Cr-Substitution in Ba2In2O5 \mbox⋅ (H2O)x (x \textequals 0.16, 0.74)

Yoon, S., Son, K., Hagemann, H., Widenmeyer, M., Weidenkaff, A.

{Solid State Sciences}, 73, pages: 1-6, Elsevier Masson SAS, Paris, 2017 (article)

DOI [BibTex]

DOI [BibTex]


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Comment on half-integer quantum numbers for the total angular momentum of photons in light beams with finite lateral extensions

Fähnle, M.

{American Journal of Modern Physics}, 6(5):88-90, Science Publishing Group, New York, NY, 2017 (article)

DOI [BibTex]

DOI [BibTex]


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Unifying ultrafast demagnetization and intrinsic Gilbert damping in Co/Ni bilayers with electronic relaxation near the Fermi surface

Zhang, W., He, W., Zhang, X.-Q., Cheng, Z.-H., Teng, J., Fähnle, M.

{Physical Review B}, 96(22), American Physical Society, Woodbury, NY, 2017 (article)

DOI [BibTex]

DOI [BibTex]


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Influence of the skin barrier on the penetration of topically-applied dexamethasone probed by soft X-ray spectromicroscopy

Yamamoto, K., Klossek, A., Flesch, R., Rancan, F., Weigand, M., Bykova, I., Bechtel, M., Ahlberg, S., Vogt, A., Blume-Peytavi, U., Schrade, P., Bachmann, S., Hedtrich, S., Schäfer-Korting, M., Rühl, E.

{European Journal of Pharmaceutics and Biopharmaceutics}, 118, pages: 30-37, Elsevier, Amsterdam, 2017 (article)

DOI [BibTex]

DOI [BibTex]


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Capture of heavy hydrogen isotopes in a metal-organic framework with active Cu(I) sites

Weinrauch, I., Savchenko, I., Denysenko, D., Souliou, S. M., Kim, H., Le Tacon, M., Daemen, L. L., Cheng, Y., Mavrandonakis, A., Ramirez-Cuesta, A. J., Volkmer, D., Schütz, G., Hirscher, M., Heine, T.

{Nature Communications}, 8, Nature Publishing Group, London, 2017 (article)

DOI [BibTex]

DOI [BibTex]


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Multiscale simulations of topological transformations in magnetic-skyrmion spin structures

De Lucia, A., Litzius, K., Krüger, B., Tretiakov, O. A., Kläui, M.

{Physical Review B}, 96(2), American Physical Society, Woodbury, NY, 2017 (article)

DOI [BibTex]

DOI [BibTex]


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Unexpectedly marginal effect of electronic correlations on ultrafast demagnetization after femtosecond laser-pulse excitation

Weng, W., Huang, Haonan, Briones Paz, J. Z., Teeny, N., Müller, B. Y., Haag, M., Kuhn, T., Fähnle, M.

{Physical Review B}, 95(22), American Physical Society, Woodbury, NY, 2017 (article)

DOI [BibTex]

DOI [BibTex]


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Black manganese-rich crusts on a Gothic cathedral

Macholdt, D. S., Herrmann, S., Jochum, K. P., Kilcoyne, A. L. D., Laubscher, T., Pfisterer, H. K., Pöhlker, C., Schwager, B., Weber, B., Weigand, M., Domke, K. F., Andreae, M. O.

{Atmospheric Environment}, 171, pages: 205-220, Elsevier, Amsterdam [u.a.], 2017 (article)

DOI [BibTex]

DOI [BibTex]

2011


The Oxidation of Fe(111)
The Oxidation of Fe(111)

Davies, R., Edwards, D., Gräfe, J., Gilbert, L., Davies, P., Hutchings, G., Bowker, M.

Surface Science, 605(17-18):1754-1762, 2011 (article)

Abstract
The oxidation of Fe(111) was studied using Auger electron spectroscopy (AES), low energy electron diffraction (LEED), X-ray photoelectron spectroscopy (XPS), ion scattering spectroscopy (ISS) and scanning tunnelling microscopy (STM). Oxidation of the crystal was found to be a very fast process, even at 200 K, and the Auger O signal saturation level is reached within ~ 50 × 10− 6 mbar s. Annealing the oxidised surface at 773 K causes a significant decline in apparent surface oxygen concentration and produces a clear (6 × 6) LEED pattern, whereas after oxidation at ambient temperature no pattern was observed. STM results indicate that the oxygen signal was reduced due to the nucleation of large, but sparsely distributed oxide islands, leaving mainly the smooth (6 × 6) structure between the islands. The reactivity of the (6 × 6) layer towards methanol was investigated using temperature programmed desorption (TPD), which showed mainly decomposition to CO and CO2, due to the production of formate intermediates on the surface. Interestingly, this removes the (6 × 6) structure by reduction, but it can be reformed from the sink of oxygen present in the large oxide islands simply by annealing at 773 K for a few minutes. The (6 × 6) appears to be a relatively stable, pseudo-oxide phase, that may be useful as a model oxide surface.

DOI [BibTex]

2011

DOI [BibTex]


High-resolution x-ray absorption spectroscopy of BaTiO${}_{3}$: Experiment and first-principles calculations
High-resolution x-ray absorption spectroscopy of BaTiO_3: Experiment and first-principles calculations

Chassé, A., Borek, S., Schindler, K., Trautmann, M., Huth, M., Steudel, F., Makhova, L., Gräfe, J., Denecke, R.

Physical Review B, 84, pages: 195135, 2011 (article)

Abstract
High resolution x-ray absorption spectroscopy (XAS) affords new insight into the microscopic properties of perovskite transition metal oxides. Interpretation of XAS spectra in transition metal oxides requires theoretical tools capable of describing relativistic and many-body effects. In this work, full relativistic (SPR-KKR) and multiplet calculations (CTM4XAS) are carried out and compared to experimental multiedge XAS spectra of BaTiO3 single crystals. The impact of relativistic and many-body effects on the calculated density of states and x-ray absorption near edge structure spectra are individually considered.

DOI [BibTex]

DOI [BibTex]


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Electron theory of fast and ultrafast dissipative magnetization dynamics

Fähnle, M., Illg, C.

{Journal of Physics: Condensed Matter}, 23, 2011 (article)

DOI [BibTex]

DOI [BibTex]


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Large-area hard magnetic L10-FePt nanopatterns by nanoimprint lithography

Bublat, T., Goll, D.

{Nanotechnology}, 22(31), 2011 (article)

DOI [BibTex]


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Hydrogen storage by cryoadsorption in ultrahigh-porosity metal-organic frameworks

Hirscher, M.

{Angewandte Chemie International Edition}, 50(3):581-582, 2011 (article)

DOI [BibTex]

DOI [BibTex]


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Multilayer Fresnel zone plate for soft X-ray microscopy resolves sub-39 nm structures

Mayer, M., Grévent, C., Szeghalmi, A., Knez, M., Weigand, M., Rehbein, S., Schneider, G., Baretzky, B., Schütz, G.

{Ultramicroscopy}, 111, pages: 1706-1711, 2011 (article)

DOI [BibTex]

DOI [BibTex]


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Generalized Gilbert equation including inertial damping: derivation from an extended breathing Fermi surface model

Fähnle, M., Steiauf, D., Illg, C.

{Physical Review B}, 84, 2011 (article)

DOI [BibTex]


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Hydrogen physisorption in high SSA microporous materials - A comparison between AX-21\textunderscore33 and MOF-177 at cryogenic conditions

Schlichtenmayer, M., Streppel, B., Hirscher, M.

{International Journal of Hydrogen Energy}, 36, pages: 586-591, 2011 (article)

DOI [BibTex]

DOI [BibTex]


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Magnetic vortex core reversal by excitation of spin waves

Kammerer, M., Weigand, M., Curcic, M., Noske, M., Sproll, M., Vansteenkiste, A., Van Waeyenberge, B., Stoll, H., Woltersdorf, G., Back, C. H., Schütz, G.

{Nature Communications}, 2, pages: 279-284, 2011 (article)

DOI [BibTex]

DOI [BibTex]


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Magnetism studied with circularly polarized X-rays

Schütz, G., Goering, E., Stoll, H.

{International Journal of Materials Research}, 102(7):773-783, 2011 (article)

DOI [BibTex]

DOI [BibTex]


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Coupled vortex oscillations in spatially separated permalloy squares

Vogel, A., Kamionka, T., Martens, M., Drews, A., Chou, K., Tyliszczak, T., Stoll, H., Van Waeyenberge, B., Meier, G.

{Physical Review Letters}, 106, 2011 (article)

DOI [BibTex]

DOI [BibTex]


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Contruction of basis functions with crystal symmetry for the spin-cluster expansion of the magnetic energy on the atomic scale

Dietermann, F., Singer, R., Fähnle, M.

{Journal of Mathematical Physics}, 52, 2011 (article)

DOI [BibTex]

DOI [BibTex]


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Magnetic patterning perpendicular anisotropy FePd alloy films by masked ion irradiation

Merkel, D. G., Bottyán, L., Tanczikó, F., Zolnai, Z., Nagy, N., Vértesy, G., Waizinger, J., Bommer, L.

{Journal of Applied Physics}, 109(12), 2011 (article)

DOI [BibTex]

DOI [BibTex]


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Stability of the current-carrying state in nonhomogeneous MgB2 films

Treiber, S., Stahl, C., Schütz, G., Albrecht, J.

{Physical Review B}, 84, 2011 (article)

DOI [BibTex]

DOI [BibTex]


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Orbital reflectometry of oxide heterostructures

Benckiser, E., Haverkort, M. W., Brück, S., Goering, E., Macke, S., Fraño, A., Yang, X., Andersen, O. K., Cristiani, G., Habermeier, H., Boris, A. V., Zegkinoglou, I., Wochner, P., Kim, H., Hinkov, V., Keimer, B.

{Nature Materials}, 10(3):189-193, 2011 (article)

DOI [BibTex]

DOI [BibTex]


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Potential explanation of charge response of magnetization in nanoporous systems

Subkow, S., Fähnle, M.

{Physical Review B}, 84, 2011 (article)

DOI [BibTex]

DOI [BibTex]


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Large hidden orbital moments in magnetite

Goering, E.

{Physica Status Solidi B}, 248(10):2345-2351, 2011 (article)

DOI [BibTex]

DOI [BibTex]


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Cr magnetization reversal at the CrO2/RuO2 interface: Origin of the reduced GMR effect

Zafar, K., Audehm, P., Schütz, G., Goering, E., Pathak, M., Chetry, K. B., LeClair, P. R., Gupta, A.

{Physical Review B}, 84, 2011 (article)

DOI [BibTex]

DOI [BibTex]


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Magnetocaloric effect, magnetic domain structure and spin-reorientation transitios in HoCo5 single crystals

Skokov, K. P., Pastushenkov, Y. G., Koshkid\textquotesingleko, Y. S., Schütz, G., Goll, D., Ivanova, T. I., Nikitin, S. A., Semenova, E. M., Petrenko, A. V.

{Journal of Magnetism and Magnetic Materials}, 323(5):447-450, 2011 (article)

DOI [BibTex]

DOI [BibTex]


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Elucidating gating effects for hydrogen sorption in MFU-4-type triazolate-based metal-organic frameworks featuring different pore sizes

Denysenko, D., Grzywa, M., Tonigold, M., Streppel, B., Krkljus, I., Hirscher, M., Mugnaioli, E., Kolb, U., Hanss, J., Volkmer, D.

{Chemistry - A European Journal}, 17(6):1837-1848, 2011 (article)

DOI [BibTex]

DOI [BibTex]


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BET specific surface area and pore structure of MOFs determined by hydrogen adsorption at 20 K

Streppel, B., Hirscher, M.

{Physical Chemistry Chemical Physics}, 13(8):3220-3222, 2011 (article)

DOI [BibTex]

DOI [BibTex]


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High contrast magnetic and nonmagnetic sample current microscopy for bulk and transparent samples using soft X-rays

Nolle, D., Weigand, M., Schütz, G., Goering, E.

{Microscopy and Microanalysis}, 17, pages: 834-842, 2011 (article)

DOI [BibTex]