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2019


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Superior magnetic performance in FePt L10 nanomaterials

Son, K., Ryu, G. H., Jeong, H., Fink, L., Merz, M., Nagel, P., Schuppler, S., Richter, G., Goering, E., Schütz, G.

{Small}, 15(34), Wiley, Weinheim, Germany, 2019 (article)

DOI [BibTex]

2019

DOI [BibTex]


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Niobium near-surface composition during nitrogen infusion relevant for superconducting radio-frequency cavities

Semione, G. D. L., Dangwal Pandey, A., Tober, S., Pfrommer, J., Poulain, A., Drnec, J., Schütz, G., Keller, T. F., Noei, H., Vonk, V., Foster, B., Stierle, A.

{Physical Review Accelerators and Beams}, 22(10), American Physical Society, Ridge, NY, USA, 2019 (article)

DOI [BibTex]

DOI [BibTex]


{Vizualizing nanoscale spin waves using MAXYMUS}
Vizualizing nanoscale spin waves using MAXYMUS

Gräfe, J., Weigand, M., Van Waeyenberge, B., Gangwar, A., Groß, F., Lisiecki, F., Rychly, J., Stoll, H., Träger, N., Förster, J., Stobiecki, F., Dubowik, J., Klos, H., Krwaczyk, M., Back, C. H., Goering, E. J., Schütz, G.

{Proceedings of SPIE}, 11090, SPIE, Bellingham, Washington, 2019 (article)

Abstract
Magnonics research, i.e. the manipulation of spin waves for information processing, is a topic of intense research interest in the past years. FMR, BLS and MOKE measurements lead to tremendous success and advancement of the field. However, these methods are limited in their spatial resolution. X-ray microscopy opens up a way to push to spatial resolutions below 100 nm. Here, we discuss the methodology of STXM for pump-probe data acquisition with single photon counting and arbitrary excitation patterns. Furthermore, we showcase these capabilities using two magnonic crystals as examples: an antidot lattice and a Fibonacci quasicrystal.

DOI [BibTex]

DOI [BibTex]


{Interpreting first-order reversal curves beyond the Preisach model: An experimental permalloy microarray investigation}
Interpreting first-order reversal curves beyond the Preisach model: An experimental permalloy microarray investigation

Groß, F., Ilse, S. E., Schütz, G., Gräfe, J., Goering, E.

{Physical Review B}, 99(6), American Physical Society, Woodbury, NY, 2019 (article)

Abstract
First-order reversal curves (FORCs) are a powerful tool to separate microscopic coercivities and interactions in a system without the need for lateral resolution. However, measured FORC densities are not always straightforward to interpret, especially if the system is interaction dominated and the Preisach-like interpretation of the FORC density breaks down. This is why FORC is often seen as a magnetic fingerprint instead of a measurement method yielding quantitative information. To understand additional features arising from the interactions in the system, we purposely designed permalloy microstructures which violate the Mayergoyz criteria. These artificial systems allow us to isolate the origin of an additional interaction peak in the FORC density. Modeling the system as a superposition of dipoles allows us to extract interaction strength parameters from this static simulation. Additionally, we suggest a linear relation between integrated interaction peak volume and interaction strength within the system. The presented correlation could be used to investigate the interaction behavior of samples as a function of structural parameters within a series of FORC measurements. This is an important step towards a more quantitative understanding of FORCs which violate the Mayergoyz criteria and away from a fingerprint interpretation.

DOI [BibTex]


Bistability of magnetic states in Fe-Pd nanocap arrays
Bistability of magnetic states in Fe-Pd nanocap arrays

Aravind, P. B., Heigl, M., Fix, M., Groß, F., Gräfe, J., Mary, A., Rajgowrav, C. R., Krupiński, M., Marszałek, M., Thomas, S., Anantharaman, M. R., Albrecht, M.

Nanotechnology, 30, pages: 405705, 2019 (article)

Abstract
Magnetic bistability between vortex and single domain states in nanostructures are of great interest from both fundamental and technological perspectives. In soft magnetic nanostructures, the transition from a uniform collinear magnetic state to a vortex state (or vice versa) induced by a magnetic field involves an energy barrier. If the thermal energy is large enough for overcoming this energy barrier, magnetic bistability with a hysteresis-free switching occurs between the two magnetic states. In this work, we tune this energy barrier by tailoring the composition of FePd alloys, which were deposited onto self-assembled particle arrays forming magnetic vortex structures on top of the particles. The bifurcation temperature, where a hysteresis-free transition occurs, was extracted from the temperature dependence of the annihilation and nucleation field which increases almost linearly with Fe content of the magnetic alloy. This study provides insights into the magnetization reversal process associated with magnetic bistability, which allows adjusting the bifurcation temperature range by the material properties of the nanosystem.

link (url) [BibTex]

link (url) [BibTex]


Anatomy of Skyrmionic Textures in Magnetic Multilayers
Anatomy of Skyrmionic Textures in Magnetic Multilayers

Li, W., Bykova, I., Zhang, S., Yu, G., Tomasello, R., Carpentieri, M., Liu, Y., Guang, Y., Gräfe, J., Weigand, M., Burn, D. M., Laan, G. V. D., Hesjedal, T., Yan, Z., Feng, J., Wan, C., Wei, J., Wang, X., Zhang, X., Xu, H., Guo, C., Wei, H., Finocchio, G., Han, X., Schütz, G.

Advanced Materials, 31, pages: 1807683, 2019 (article)

Abstract
Room temperature magnetic skyrmions in magnetic multilayers are considered as information carriers for future spintronic applications. Currently, a detailed understanding of the skyrmion stabilization mechanisms is still lacking in these systems. To gain more insight, it is first and foremost essential to determine the full real‐space spin configuration. Here, two advanced X‐ray techniques are applied, based on magnetic circular dichroism, to investigate the spin textures of skyrmions in [Ta/CoFeB/MgO]n multilayers. First, by using ptychography, a high‐resolution diffraction imaging technique, the 2D out‐of‐plane spin profile of skyrmions with a spatial resolution of 10 nm is determined. Second, by performing circular dichroism in resonant elastic X‐ray scattering, it is demonstrated that the chirality of the magnetic structure undergoes a depth‐dependent evolution. This suggests that the skyrmion structure is a complex 3D structure rather than an identical planar texture throughout the layer stack. The analyses of the spin textures confirm the theoretical predictions that the dipole–dipole interactions together with the external magnetic field play an important role in stabilizing sub‐100 nm diameter skyrmions and the hybrid structure of the skyrmion domain wall. This combined X‐ray‐based approach opens the door for in‐depth studies of magnetic skyrmion systems, which allows for precise engineering of optimized skyrmion heterostructures.

link (url) DOI [BibTex]

link (url) DOI [BibTex]


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The route to supercurrent transparent ferromagnetic barriers in superconducting matrix

Ivanov, Y. P., Soltan, S., Albrecht, J., Goering, E., Schütz, G., Zhang, Z., Chuvilin, A.

{ACS Nano}, 13(5):5655-5661, American Chemical Society, Washington, DC, 2019 (article)

DOI [BibTex]

DOI [BibTex]


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Systematic experimental study on quantum sieving of hydrogen isotopes in metal-amide-imidazolate frameworks with narrow 1-D channels

Mondal, S. S., Kreuzer, A., Behrens, K., Schütz, G., Holdt, H., Hirscher, M.

{ChemPhysChem}, 20(10):1311-1315, Wiley-VCH, Weinheim, Germany, 2019 (article)

DOI [BibTex]

DOI [BibTex]


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Exploiting dynamic opening of apertures in a partially fluorinated MOF for enhancing H2 desorption temperature and isotope separation

Zhang, L., Jee, S., Park, J., Jung, M., Wallcher, D., Franz, A., Lee, W., Yoon, M., Choi, K., Hirscher, M., Oh, H.

{Journal of the American Chemical Society}, 141(50):19850-19858, American Chemical Society, Washington, DC, 2019 (article)

DOI [BibTex]

DOI [BibTex]


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Speeding up the extended Kalman filter approach for denoising XMCD movies of fast magnetization dynamics

Fähnle, M., Schütz, G.

{Ultramicroscopy}, 206, North-Holland, Amsterdam, 2019 (article)

DOI [BibTex]


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Artifacts from manganese reduction in rock samples prepared by focused ion beam (FIB) slicing for X-ray microspectroscopy

Macholdt, D. S., Förster, J., Müller, M., Weber, B., Kappl, M., Kilcoyne, A. L. D., Weigand, M., Leitner, J., Jochum, K. P., Pöhlker, C., Andreae, M. O.

{Geoscientific instrumentation, methods and data systems}, 8(1):97-111, Copernicus Publ., Göttingen, 2019 (article)

DOI [BibTex]

DOI [BibTex]


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Magnetic field dependence of mangetotransport properties of MgB2/CrO2 bilayer thin films

Alzayed, N. S., Shahabuddin, M., Ramey, S. M., Soltan, S.

{Journal of Superconductivity and Novel Magnetism}, 32(8):2447-2455, Springer Science + Business Media B.V., New York, 2019 (article)

DOI [BibTex]

DOI [BibTex]


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Mixed-state magnetotransport properties of MgB2 thin film prepared by pulsed laser deposition on an Al2O3 substrate

Alzayed, N. S., Shahabuddin, M., Ramey, S. M., Soltan, S.

{Journal of Materials Science: Materials in Electronics}, 30(2):1547-1552, Springer, Norwell, MA, 2019 (article)

DOI [BibTex]

DOI [BibTex]


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Concepts for improving hydrogen storage in nanoporous materials

Broom, D. P., Webb, C. J., Fanourgakis, G. S., Froudakis, G. E., Trikalitis, P. N., Hirscher, M.

{International Journal of Hydrogen Energy}, 44(15):7768-7779, Elsevier, Amsterdam, 2019 (article)

DOI [BibTex]

DOI [BibTex]


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Comparison of theories of fast and ultrafast magnetization dynamics

Fähnle, M.

{Journal of Magnetism and Magnetic Materials}, 469, pages: 28-29, NH, Elsevier, Amsterdam, 2019 (article)

DOI [BibTex]

DOI [BibTex]


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Controlling dislocation nucleation-mediatd plasticity in nanostructures via surface modification

Shin, J., Chen, L. Y., Sanli, U. T., Richter, G., Labat, S., Richard, M., Cornelius, T., Thomas, O., Gianola, D. S.

{Acta Materialia}, 166, pages: 572-586, Elsevier Science, Kidlington, 2019 (article)

DOI [BibTex]

DOI [BibTex]


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Reprogrammability and scalability of magnonic Fibonacci quasicrystals

Lisiecki, F., Rychly, J., Kuswik, P., Glowinski, H., Klos, J. W., Groß, F., Bykova, I., Weigand, M., Zelent, M., Goering, E. J., Schütz, G., Gubbiotti, G., Krawczyk, M., Stobiecki, F., Dubowik, J., Gräfe, J.

{Physical Review Applied}, 11(5), American Physical Society, College Park, Md. [u.a.], 2019 (article)

DOI [BibTex]

DOI [BibTex]

2017


{Temperature-dependent first-order reversal curve measurements on unusually hard magnetic low-temperature phase of MnBi}
Temperature-dependent first-order reversal curve measurements on unusually hard magnetic low-temperature phase of MnBi

Muralidhar, S., Gräfe, J., Chen, Y., Etter, M., Gregori, G., Ener, S., Sawatzki, S., Hono, K., Gutfleisch, O., Kronmüller, H., Schütz, G., Goering, E. J.

{Physical Review B}, 95(2), American Physical Society, Woodbury, NY, 2017 (article)

Abstract
We have performed first-order reversal curve (FORC) measurements to investigate the irreversible magnetization processes in the low-temperature phase of MnBi. Using temperature-dependent FORC analysis, we are able to provide a clear insight into the effects of microstructural parameters such as grain diameter, shape, and surface composition on the coercivity of nucleation hardened permanent magnet MnBi. FORC diagrams of MnBi show a unique broadening and narrowing of the coercive field distribution with increasing temperature. We were able to microscopically identify the reason for this behavior, based on the shift in the single domain critical diameter from nearly 1 to 2 μm, thereby changing the dependence of coercivity with particle size. This is based on a strong increase in the uniaxial anisotropy constant with increasing temperature. Furthermore, the results also give an additional confirmation that the magnetic hardening in low-temperature phase MnBi occurs due to nucleation mechanisms. In our case, we show that temperature-dependent FORC measurements provide a powerful tool for the microscopic understanding of high-performance permanent magnet systems.

DOI Project Page [BibTex]

2017

DOI Project Page [BibTex]


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Exploiting diffusion barrier and chemical affinity of metal-organic frameworks for efficient hydrogen isotope separation

Kim, J. Y., Balderas-Xicohténcatl, R., Zhang, L., Kang, S. G., Hirscher, M., Oh, H., Moon, H. R.

{Journal of the American Chemical Society}, 139(42):15135-15141, American Chemical Society, Washington, DC, 2017 (article)

DOI [BibTex]

DOI [BibTex]


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Facile fabrication of mesoporous silica micro-jets with multi-functionalities

Vilela, D., Hortelao, A. C., Balderas-Xicohténcatl, R., Hirscher, M., Hahn, K., Ma, X., Sánchez, S.

{Nanoscale}, 9(37):13990-13997, Royal Society of Chemistry, Cambridge, UK, 2017 (article)

DOI [BibTex]

DOI [BibTex]


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Functionalised metal-organic frameworks: a novel approach to stabilising single metal atoms

Szilágyi, P. Á., Rogers, D. M., Zaiser, I., Callini, E., Turner, S., Borgschulte, A., Züttel, A., Geerlings, H., Hirscher, M., Dam, B.

{Journal of Materials Chemistry A}, 5(30):15559-15566, Royal Society of Chemistry, Cambridge, UK, 2017 (article)

DOI [BibTex]

DOI [BibTex]


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Selective hydrogen isotope separation via breathing transition in MIL-53(Al)

Kim, J. Y., Zhang, L., Balderas-Xicohténcatl, R., Park, J., Hirscher, M., Moon, H. R., Oh, H.

{Journal of the American Chemical Society}, 139(49):17743-17746, American Chemical Society, Washington, DC, 2017 (article)

DOI [BibTex]

DOI [BibTex]


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Efficient synthesis for large-scale production and characterization for hydrogen storage of ligand exchanged MOF-74/174/184-M (M\textequalsMg2+, Ni2+)

Oh, H., Maurer, S., Balderas-Xicohténcatl, R., Arnold, L., Magdysyuk, O. V., Schütz, G., Müller, U., Hirscher, M.

{International Journal of Hydrogen Energy}, 42(2):1027-1035, Elsevier, Amsterdam, 2017 (article)

DOI [BibTex]

DOI [BibTex]


{Advanced magneto-optical Kerr effect measurements of superconductors at low temperatures}
Advanced magneto-optical Kerr effect measurements of superconductors at low temperatures

Stahl, C., Gräfe, J., Ruoß, S., Zahn, P., Bayer, J., Simmendinger, J., Schütz, G., Albrecht, J.

{AIP Advances}, 7(10), 2017 (article)

Abstract
Magneto-optical Kerr-effect (MOKE) measurements of superconducting films with soft-magnetic coatings are performed at low temperatures using a laser-based MOKE set-up. An elaborate measurement scheme with internal reference allows the quantitative comparison of the temperature dependent Kerr-amplitude with the magnetic field generated by supercurrents. For this purpose, an amorphous CoFeB thin film exhibiting a large Kerr-signal is deposited directly on top of the YBCO superconductor acting as field sensing layer. It is shown that the resulting magnetic hysteresis loops of the soft-magnetic film can be used to reconstruct the electric properties of the superconductor.

DOI [BibTex]

DOI [BibTex]


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Corrosion-protected hybrid nanoparticles

Jeong, H., Alarcón-Correa, M., Mark, A. G., Son, K., Lee, T., Fischer, P.

{Advanced Science}, 4(12), Wiley-VCH, Weinheim, 2017 (article)

DOI [BibTex]

DOI [BibTex]


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Investigation of the Dzyaloshinskii-Moriya interaction and room temperature skyrmions in W/CoFeB/MgO thin films and microwires

Jaiswal, S., Litzius, K., Lemesh, I., Büttner, F., Finizio, S., Raabe, J., Weigand, M., Lee, K., Langer, J., Ocker, B., Jakob, G., Beach, G. S. D., Kläui, M.

{Applied Physics Letters}, 111(2), American Institute of Physics, Melville, NY, 2017 (article)

DOI [BibTex]

DOI [BibTex]


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Ultrafast demagnetization after femtosecond laser pulses: Transfer of angular momentum from the electronic system to magnetoelastic spin-phonon modes

Fähnle, M., Tsatsoulis, T., Illg, C., Haag, M., Müller, B. Y., Zhang, L.

{Journal of Superconductivity and Novel Magnetism}, 30(5):1381-1387, Springer Science + Business Media B.V., New York, 2017 (article)

DOI [BibTex]

DOI [BibTex]


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Magnetic behavior of single chain magnets in metal organic frameworks CPO-27-Co

Son, K., Goering, E., Hirscher, M., Oh, H.

{Journal of Nanoscience and Nanotechnology}, 17(10):7541-7546, American Scientific Publishers, Stevenson Ranch, Calif., 2017 (article)

DOI [BibTex]

DOI [BibTex]


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Switching by domain-wall automotion in asymmetric ferromagnetic rings

Mawass, M., Richter, K., Bisig, A., Reeve, R. M., Krüger, B., Weigand, M., Stoll, H., Krone, A., Kronast, F., Schütz, G., Kläui, M.

{Physical Review Applied}, 7(4), American Physical Society, College Park, Md. [u.a.], 2017 (article)

DOI [BibTex]

DOI [BibTex]


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A neutral atom moving in an external magnetic field does not feel a Lorentz force

Fähnle, M.

{American Journal of Modern Physics}, 6(6):153-155, Science Publishing Group, New York, NY, 2017 (article)

DOI [BibTex]

DOI [BibTex]


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Adsorption von Wasserstoffmolekülen in nanoporösen Gerüststrukturen

Kotzur, Nadine

Universität Stuttgart, Stuttgart, 2017 (mastersthesis)

[BibTex]

[BibTex]


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Smooth and rapid microwave synthesis of MIL-53(Fe) including superparamagnetic \textlessgamma\textgreater-Fe2O3 nanoparticles

Wengert, S., Albrecht, J., Ruoß, S., Stahl, C., Schütz, G., Schäfer, R.

{Journal of Magnetism and Magnetic Materials}, 444, pages: 168-172, NH, Elsevier, Amsterdam, 2017 (article)

DOI [BibTex]

DOI [BibTex]


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Characterization and differentiation of rock varnish types from different environments by microanalytical techniques

Macholdt, D. S., Jochum, K. P., Pöhlker, C., Arangio, A., Förster, J., Stoll, B., Weis, U., Weber, B., Müller, M., Kappl, M., Shiraiwa, M., Kilcoyne, A. L. D., Weigand, M., Scholz, D., Haug, G. H., Al-Amri, A., Andreae, M. O.

{Chemical Geology}, 459, pages: 91-118, Elsevier, Amsterdam, 2017 (article)

DOI [BibTex]

DOI [BibTex]


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Skyrmion Hall effect revealed by direct time-resolved X-ray microscopy

Litzius, K., Lemesh, I., Krüger, B., Bassirian, P., Caretta, L., Richter, K., Büttner, F., Sato, K., Tretiakov, O. A., Förster, J., Reeve, R. M., Weigand, M., Bykova, I., Stoll, H., Schütz, G., Beach, G. S. D., Kläui, M.

{Nature Physics}, 13(2):170-175, Nature Pub. Group, London, 2017 (article)

DOI [BibTex]

DOI [BibTex]


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Comment on magnonic black holes

Fähnle, M., Schütz, G.

{Journal of Magnetism and Magnetic Materials}, 444, pages: 146-146, NH, Elsevier, Amsterdam, 2017 (article)

DOI [BibTex]

DOI [BibTex]


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Cr-Substitution in Ba2In2O5 \mbox⋅ (H2O)x (x \textequals 0.16, 0.74)

Yoon, S., Son, K., Hagemann, H., Widenmeyer, M., Weidenkaff, A.

{Solid State Sciences}, 73, pages: 1-6, Elsevier Masson SAS, Paris, 2017 (article)

DOI [BibTex]

DOI [BibTex]


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Comment on half-integer quantum numbers for the total angular momentum of photons in light beams with finite lateral extensions

Fähnle, M.

{American Journal of Modern Physics}, 6(5):88-90, Science Publishing Group, New York, NY, 2017 (article)

DOI [BibTex]

DOI [BibTex]


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Unifying ultrafast demagnetization and intrinsic Gilbert damping in Co/Ni bilayers with electronic relaxation near the Fermi surface

Zhang, W., He, W., Zhang, X.-Q., Cheng, Z.-H., Teng, J., Fähnle, M.

{Physical Review B}, 96(22), American Physical Society, Woodbury, NY, 2017 (article)

DOI [BibTex]

DOI [BibTex]


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Influence of the skin barrier on the penetration of topically-applied dexamethasone probed by soft X-ray spectromicroscopy

Yamamoto, K., Klossek, A., Flesch, R., Rancan, F., Weigand, M., Bykova, I., Bechtel, M., Ahlberg, S., Vogt, A., Blume-Peytavi, U., Schrade, P., Bachmann, S., Hedtrich, S., Schäfer-Korting, M., Rühl, E.

{European Journal of Pharmaceutics and Biopharmaceutics}, 118, pages: 30-37, Elsevier, Amsterdam, 2017 (article)

DOI [BibTex]

DOI [BibTex]


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Capture of heavy hydrogen isotopes in a metal-organic framework with active Cu(I) sites

Weinrauch, I., Savchenko, I., Denysenko, D., Souliou, S. M., Kim, H., Le Tacon, M., Daemen, L. L., Cheng, Y., Mavrandonakis, A., Ramirez-Cuesta, A. J., Volkmer, D., Schütz, G., Hirscher, M., Heine, T.

{Nature Communications}, 8, Nature Publishing Group, London, 2017 (article)

DOI [BibTex]

DOI [BibTex]


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Multiscale simulations of topological transformations in magnetic-skyrmion spin structures

De Lucia, A., Litzius, K., Krüger, B., Tretiakov, O. A., Kläui, M.

{Physical Review B}, 96(2), American Physical Society, Woodbury, NY, 2017 (article)

DOI [BibTex]

DOI [BibTex]


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Unexpectedly marginal effect of electronic correlations on ultrafast demagnetization after femtosecond laser-pulse excitation

Weng, W., Huang, Haonan, Briones Paz, J. Z., Teeny, N., Müller, B. Y., Haag, M., Kuhn, T., Fähnle, M.

{Physical Review B}, 95(22), American Physical Society, Woodbury, NY, 2017 (article)

DOI [BibTex]

DOI [BibTex]


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Black manganese-rich crusts on a Gothic cathedral

Macholdt, D. S., Herrmann, S., Jochum, K. P., Kilcoyne, A. L. D., Laubscher, T., Pfisterer, H. K., Pöhlker, C., Schwager, B., Weber, B., Weigand, M., Domke, K. F., Andreae, M. O.

{Atmospheric Environment}, 171, pages: 205-220, Elsevier, Amsterdam [u.a.], 2017 (article)

DOI [BibTex]

DOI [BibTex]

2015


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Isosteric heat of hydrogen adsorption on MOFs: comparison between adsorption calorimetry, sorption isosteric metod, and analytical models

Kloutse, A. F., Zacharia, R., Cossement, D., Chahine, R., Balderas-Xicohténcatl, R., Oh, H., Streppel, B., Schlichtenmayer, M., Hirscher, M.

{Applied Physics A}, 121(4):1417-1424, Springer-Verlag Heidelberg, Heidelberg, 2015 (article)

DOI [BibTex]

2015

DOI [BibTex]